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Observation of high-energy vibrational overtones of molecules in solids: Local modes and intramolecular relaxations

Perry, J. W. and Zewail, A. H. (1979) Observation of high-energy vibrational overtones of molecules in solids: Local modes and intramolecular relaxations. Journal of Chemical Physics, 70 (1). pp. 582-584. ISSN 0021-9606. http://resolver.caltech.edu/CaltechAUTHORS:PERjcp79

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Abstract

In the last few years, the spectra of vibrational overtones (1) (at ~15-20,000 cm^-1) in large molecules have received considerable attention. The focus is on three problems dealing with the origin of relaxation at such high energies, the association of spectral band positions with the local modes (LM) in molecules, and the relevance of these spectra to possible selectivity in laser-induced chemistry.


Item Type:Article
Additional Information:© 1979 American Institute of Physics. Received 15 September 1978. [A.H.Z. was an] Alfred P. Sloan Fellow. Arthur Amos Noyes Laboratory of Chemical Physics, Contribution No. 5886. This work is supported by a grant from the National Science Foundation.
Record Number:CaltechAUTHORS:PERjcp79
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:PERjcp79
Alternative URL:http://dx.doi.org/10.1063/1.437176
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:10649
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:01 Jun 2008
Last Modified:26 Dec 2012 10:03

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