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Diffusion kinetics in radiation chemistry. I. Generalized formulation and criticism of diffusion model

Kuppermann, Aron and Belford, Geneva G. (1962) Diffusion kinetics in radiation chemistry. I. Generalized formulation and criticism of diffusion model. Journal of Chemical Physics, 36 (6). pp. 1412-1426. ISSN 0021-9606. http://resolver.caltech.edu/CaltechAUTHORS:KUPjcp62a

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Abstract

A generalized formulation of the diffusion-kinetic model of track effects in radiation chemistry is presented and criticized. It permits consideration of complex mechanisms, arbitrary initial distributions and radical correlation effects. Methods for the numerical integration of the associated differential equations on high-speed electronic digital computers are given and their accuracy is examined. Several applications are suggested.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1063/1.1732759DOIUNSPECIFIED
http://link.aip.org/link/?JCPSA6/36/1412/1PublisherUNSPECIFIED
Additional Information:© 1962 American Institute of Physics. Received November 30, 1959. Work partially supported by the Atomic Energy Commission. Presented in part at the 136th Meeting of the American Chemical Society in Atlantic City, September, 1959. At the referee's suggestion, publication of this paper was postponed until the second one, which follows, was ready.
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Atomic Energy CommissionUNSPECIFIED
Record Number:CaltechAUTHORS:KUPjcp62a
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:KUPjcp62a
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:11488
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:07 Sep 2008 07:00
Last Modified:26 Dec 2012 10:15

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