Kuppermann, Aron and Belford, Geneva G. (1962) Diffusion kinetics in radiation chemistry. I. Generalized formulation and criticism of diffusion model. Journal of Chemical Physics, 36 (6). pp. 1412-1426. ISSN 0021-9606. http://resolver.caltech.edu/CaltechAUTHORS:KUPjcp62a
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A generalized formulation of the diffusion-kinetic model of track effects in radiation chemistry is presented and criticized. It permits consideration of complex mechanisms, arbitrary initial distributions and radical correlation effects. Methods for the numerical integration of the associated differential equations on high-speed electronic digital computers are given and their accuracy is examined. Several applications are suggested.
|Additional Information:||© 1962 American Institute of Physics. Received November 30, 1959. Work partially supported by the Atomic Energy Commission. Presented in part at the 136th Meeting of the American Chemical Society in Atlantic City, September, 1959. At the referee's suggestion, publication of this paper was postponed until the second one, which follows, was ready.|
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|Deposited By:||Tony Diaz|
|Deposited On:||07 Sep 2008 07:00|
|Last Modified:||26 Dec 2012 10:15|
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