Chuang, Kangway V. and Navarro, Raul and Reisman, Sarah E. (2011) Short, Enantioselective Total Syntheses of (—)-8-Demethoxyrunanine and (—)-Cepharatines A, C, and D. Angewandte Chemie International Edition, 50 (40). pp. 9447-9451. ISSN 1433-7851 http://resolver.caltech.edu/CaltechAUTHORS:20111005-093543509
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All together! A unified synthetic strategy has resulted in the first enantioselective total syntheses of the natural products 8-demethoxyrunanine and cepharatines A, C, and D.
|Additional Information:||© 2011 Wiley-VCH Verlag GmbH & Co. Issue published online: 21 Sep 2011. Article first published online: 30 Aug 2011. Manuscript Received: 29 Jun 2011. We thank Dr. Michael Day and Mr. Larry Henling for X-ray crystallographic structural determination, as well as Prof. Brian Stoltz, Dr. Scott Virgil, and the Caltech Center for Catalysis and Chemical Synthesis for access to analytical equipment. Fellowship support was provided by the Gates Millennium Scholars Program (R.N.), the NIH (R.N., 1F31GM098025A) and the Amgen Scholars Program (K.V.C.). HRMS and X-ray crystallographic data were obtained on instruments purchased through awards to the California Institute of Technology by the NSF CRIF program (CHE-0639094, CHE-0541745). Financial support from the California Institute of Technology and the NSF (CAREER-1057143) is gratefully acknowledged.|
|Subject Keywords:||alkaloids; asymmetric synthesis; cepharatines; hasubanan; total synthesis|
|Official Citation:||Chuang, K. V., Navarro, R. and Reisman, S. E. (2011), Short, Enantioselective Total Syntheses of (−)-8-Demethoxyrunanine and (−)-Cepharatines A, C, and D. Angewandte Chemie International Edition, 50: 9447–9451. doi: 10.1002/anie.201104487|
|Usage Policy:||No commercial reproduction, distribution, display or performance rights in this work are provided.|
|Deposited By:||Ruth Sustaita|
|Deposited On:||05 Oct 2011 17:14|
|Last Modified:||11 Oct 2012 18:59|
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