Liu, Albert Tianxiang and Zaveri, Rahul A. and Seinfeld, John H. (2014) Analytical solution for transient partitioning and reaction of a condensing vapor species in a droplet. Atmospheric Environment, 89 . pp. 651-654. ISSN 1352-2310 . http://resolver.caltech.edu/CaltechAUTHORS:20140605-084912235
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We present the exact analytical solution of the transient equation of gas-phase diffusion of a condensing vapor to, and diffusion and reaction in, an aqueous droplet. Droplet-phase reaction is represented by first-order chemistry. The solution facilitates study of the dynamic nature of the vapor uptake process as a function of droplet size, Henry's law coefficient, and first-order reaction rate constant for conversion in the droplet phase.
|Additional Information:||© 2014 Elsevier Ltd. Received 11 December 2013; Received in revised form 25 February 2014; Accepted 28 February 2014; Available online 1 March 2014. Participation of RAZ in this study was supported by the US Department of Energy (DOE) Atmospheric System Research (ASR) Program under contract DE-AC06-76RLO 1830 at Pacific Northwest National Laboratory.|
|Subject Keywords:||Droplet; Diffusion and reaction; Henry's law constant|
|Official Citation:||Albert Tianxiang Liu, Rahul A. Zaveri, John H. Seinfeld, Analytical solution for transient partitioning and reaction of a condensing vapor species in a droplet, Atmospheric Environment, Volume 89, June 2014, Pages 651-654, ISSN 1352-2310, http://dx.doi.org/10.1016/j.atmosenv.2014.02.065. (http://www.sciencedirect.com/science/article/pii/S1352231014001617)|
|Usage Policy:||No commercial reproduction, distribution, display or performance rights in this work are provided.|
|Deposited By:||Tony Diaz|
|Deposited On:||05 Jun 2014 16:25|
|Last Modified:||05 Jun 2014 16:25|
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