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Observation of dipolar-induced spin dephasing in ionic solids using coherent optical-microwave spectroscopy

Glasbeek, M. and Hond, R. and Zewail, A. H. (1980) Observation of dipolar-induced spin dephasing in ionic solids using coherent optical-microwave spectroscopy. Physical Review Letters, 45 (9). pp. 744-747. ISSN 0031-9007. http://resolver.caltech.edu/CaltechAUTHORS:GLAprl80

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Abstract

The observation of spin dephasing in an ensemble of dipolar coupled A and B spins is reported. In CaO crystals, the A-spin species are photoexcited S=1, F22+ centers and the group of B spins consists of S=1 / 2, F+ centers. Measurements were made at different temperatures and magnetic field strengths with use of coherent optical-microwave spectroscopy. For the first time, the results show that the A-spin dephasing is influenced by exchange narrowing in the B-spin ensemble.


Item Type:Article
Additional Information:©1980 The American Physical Society. Received 2 May 1980. We wish to thank the John van Geunsfonds for the partial support of this work. One of us (A.H.Z.), an Alfred P. Sloan Fellow and Camille and Henry Dreyfus Foundation Teacher-Scholar at the Noyes Laboratory, would also like to thank the National Science Foundation for partial support of this work under Grant No. DMR-77-19478.
Record Number:CaltechAUTHORS:GLAprl80
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:GLAprl80
Alternative URL:http://dx.doi.org/10.1103/PhysRevLett.45.744
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:9184
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:19 Nov 2007
Last Modified:26 Dec 2012 09:46

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