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Electrocatalytic Oxidative Transformation of Organic Acids for Carbon–Heteroatom and Sulfur–Heteroatom Bond Formation

Li, Man and Hong, Junting and Xiao, Wei and Yang, Yang and Qiu, Di and Mo, Fanyang (2020) Electrocatalytic Oxidative Transformation of Organic Acids for Carbon–Heteroatom and Sulfur–Heteroatom Bond Formation. ChemSusChem, 13 (7). pp. 1661-1687. ISSN 1864-5631. https://resolver.caltech.edu/CaltechAUTHORS:20191216-132836799

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Abstract

The electrolysis of organic acids has garnered increasing attention in recent years. In addition to the famous electrochemical decarboxylation known as Kolbe electrolysis, a number of other electrochemical processes have been recently established that allow for the construction of carbon–heteroatom and sulfur–heteroatom bonds from organic acids. Herein, recent advances in electrochemical C−X and S−X (X=N, O, S, Se) bond‐forming reactions from five classes of organic acids and their conjugate bases, namely, carboxylic, thiocarboxylic, phosphonic, sulfinic, and sulfonic acids, are surveyed.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1002/cssc.201902657DOIArticle
ORCID:
AuthorORCID
Yang, Yang0000-0002-4956-2034
Mo, Fanyang0000-0002-4140-3020
Alternate Title:Electro-catalytic oxidative transformation of organic acids for carbon-heteroatom and sulfur-heteroatom bond formation
Additional Information:© 2019 Wilet‐VCH Verlag GmbH & Co. KGaA, Weinheim. Issue Online: 06 April 2020; Version of Record online: 21 February 2020; Accepted manuscript online: 05 December 2019; Manuscript revised: 01 December 2019; Manuscript received: 26 September 2019. This project is supported by the National Natural Science Foundation of China (grant no. 21772003 and 21933001). We also thank Peking University for a start‐up fund. This work was also partially funded by the BHP‐PKU CCUS project supported by BHP Billiton. The authors declare no conflict of interest.
Funders:
Funding AgencyGrant Number
National Natural Science Foundation of China21772003
National Natural Science Foundation of China21933001
Peking UniversityUNSPECIFIED
BHP BillitonUNSPECIFIED
Subject Keywords:electrochemistry; electrosynthesis; organic acids; oxidation; reaction mechanisms
Issue or Number:7
Record Number:CaltechAUTHORS:20191216-132836799
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20191216-132836799
Official Citation:Electrocatalytic Oxidative Transformation of Organic Acids for Carbon–Heteroatom and Sulfur–Heteroatom Bond Formation. M. Li, J. Hong, W. Xiao, Y. Yang, D. Qiu, F. Mo, ChemSusChem 2020, 13, 1661; doi: 10.1002/cssc.201902657
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:100302
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:16 Dec 2019 22:12
Last Modified:08 Apr 2020 17:04

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