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On the successes and opportunities for discovery of metal oxide photoanodes for solar fuels generators

Zhou, Lan and Shinde, Aniketa and Guevarra, Dan and Haber, Joel A. and Persson, Kristin A. and Neaton, Jeffrey B. and Gregoire, John M. (2020) On the successes and opportunities for discovery of metal oxide photoanodes for solar fuels generators. ACS Energy Letters, 5 (5). pp. 1413-1421. ISSN 2380-8195. https://resolver.caltech.edu/CaltechAUTHORS:20200331-093744929

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Abstract

The importance of metal oxide photoanodes in solar fuels technology has garnered concerted efforts in photoanode discovery in recent decades, which complement parallel efforts in development of analytical techniques and optimization strategies using standard photoanodes such as TiO₂, Fe2O₃ and BiVO₄. Theoretical guidance of high throughput experiments has been particularly effective in dramatically increasing the portfolio of metal oxide photoanodes, motivating a new era of photoanode development where the characterization and optimization techniques developed on traditional materials are applied to nascent photoanodes that exhibit visible light photoresponse. The compendium of metal oxide photoanodes presented in the present work can also serve as the basis for further technique development, with a primary goal to establish workflows for discovery of materials that perform better against the critical criteria of operational stability, visible light photoresponse, and photovoltage suitable for tandem absorber architectures.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1021/acsenergylett.0c00067DOIArticle
ORCID:
AuthorORCID
Zhou, Lan0000-0002-7052-266X
Shinde, Aniketa0000-0003-2386-3848
Guevarra, Dan0000-0002-9592-3195
Haber, Joel A.0000-0001-7847-5506
Persson, Kristin A.0000-0003-2495-5509
Neaton, Jeffrey B.0000-0001-7585-6135
Gregoire, John M.0000-0002-2863-5265
Additional Information:© 2020 American Chemical Society. Received: January 10, 2020; Accepted: March 31, 2020; Published: March 31, 2020. This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. The authors declare no competing financial interest.
Group:JCAP
Funders:
Funding AgencyGrant Number
Department of Energy (DOE)DE-SC0004993
Issue or Number:5
Record Number:CaltechAUTHORS:20200331-093744929
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20200331-093744929
Official Citation:Successes and Opportunities for Discovery of Metal Oxide Photoanodes for Solar Fuels Generators. Lan Zhou, Aniketa Shinde, Dan Guevarra, Joel A. Haber, Kristin A. Persson, Jeffrey B. Neaton, and John M. Gregoire. ACS Energy Letters 2020 5 (5), 1413-1421; DOI: 10.1021/acsenergylett.0c00067
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:102193
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:31 Mar 2020 16:50
Last Modified:11 May 2020 22:22

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