Sander, Stanley P. and Seinfeld, John H. (1976) Chemical kinetics of homogeneous atmospheric oxidation of sulfur dioxide. Environmental Science and Technology, 10 (12). pp. 1114-1123. ISSN 0013-936X. doi:10.1021/es60122a007. https://resolver.caltech.edu/CaltechAUTHORS:20200428-084748306
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Abstract
A systematic evaluation of known homogeneous SO₂ reactions which might be important in air pollution chemistry is carried out. A mechanism is developed to represent the chemistry of NO_x/hydrocarbon/SO₂ systems, and the mechanism is used to analyze available experimental data appropriate for quantitative analysis of SO₂ oxidation kinetics. Detailed comparisons of observed and predicted concentration behavior are presented. In all cases, observed SO₂ oxidation rates cannot be explained solely on the basis of those SO₂ reactions for which rate constants have been measured. The role of ozone-olefin reactions in SO₂ oxidation is elucidated.
| Item Type: | Article | ||||||
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| Additional Information: | © 1976 American Chemical Society. Received for review January 5, 1976. Accepted April 26, 1976. Work supported in part by the Jet Propulsion Laboratory and in part by National Science Foundation Grant 71ENG-02486. | ||||||
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| Issue or Number: | 12 | ||||||
| DOI: | 10.1021/es60122a007 | ||||||
| Record Number: | CaltechAUTHORS:20200428-084748306 | ||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20200428-084748306 | ||||||
| Official Citation: | Chemical kinetics of homogeneous atmospheric oxidation of sulfur dioxide. Stanley P. Sander and John H. Seinfeld. Environmental Science & Technology 1976 10 (12), 1114-1123; DOI: 10.1021/es60122a007 | ||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | ||||||
| ID Code: | 102833 | ||||||
| Collection: | CaltechAUTHORS | ||||||
| Deposited By: | Tony Diaz | ||||||
| Deposited On: | 28 Apr 2020 16:13 | ||||||
| Last Modified: | 16 Nov 2021 18:15 |
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