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Entangled light-matter interactions and spectroscopy

Szoke, Szilard and Liu, Hanzhe and Hickam, Bryce P. and He, Manni and Cushing, Scott K. (2020) Entangled light-matter interactions and spectroscopy. Journal of Materials Chemistry C, 8 (31). pp. 10732-10741. ISSN 2050-7526. https://resolver.caltech.edu/CaltechAUTHORS:20200526-082511578

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Abstract

Entangled photons exhibit non-classical light–matter interactions that create new opportunities in materials and molecular science. Notably, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one photon was present. The entangled two-photon absorption cross section approaches but does not match the one-photon absorption cross section. The entangled two-photon cross section also does not follow classical two-photon molecular design motifs. Questions such as these seed the rich but nascent field of entangled light–matter interactions. In this perspective, we use the experimental developments in entangled photon spectroscopy to outline the current status of the field. Now that the fundamental tools are outlined, it is time to start the exploration of how materials, molecules, and devices can control or utilize interactions with entangled photons.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1039/d0tc02300kDOIArticle
https://arxiv.org/abs/2004.03189arXivDiscussion Paper
ORCID:
AuthorORCID
Hickam, Bryce P.0000-0003-2120-4769
Cushing, Scott K.0000-0003-3538-2259
Additional Information:© 2020 The Royal Society of Chemistry. Submitted 13 May 2020; Accepted 19 May 2020; First published 19 May 2020. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-SC0020151. There are no conflicts to declare.
Funders:
Funding AgencyGrant Number
Department of Energy (DOE)DE-SC0020151
Issue or Number:31
Record Number:CaltechAUTHORS:20200526-082511578
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20200526-082511578
Official Citation:Entangled light-matter interactions and spectroscopy. J. Mater. Chem. C, 2020, 8, 10732-10741; doi: 10.1039/d0tc02300k
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:103436
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:26 May 2020 16:09
Last Modified:14 Aug 2020 16:59

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