Szoke, Szilard and Liu, Hanzhe and Hickam, Bryce P. and He, Manni and Cushing, Scott K. (2020) Entangled light-matter interactions and spectroscopy. Journal of Materials Chemistry C, 8 (31). pp. 10732-10741. ISSN 2050-7526. https://resolver.caltech.edu/CaltechAUTHORS:20200526-082511578
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Abstract
Entangled photons exhibit non-classical light–matter interactions that create new opportunities in materials and molecular science. Notably, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one photon was present. The entangled two-photon absorption cross section approaches but does not match the one-photon absorption cross section. The entangled two-photon cross section also does not follow classical two-photon molecular design motifs. Questions such as these seed the rich but nascent field of entangled light–matter interactions. In this perspective, we use the experimental developments in entangled photon spectroscopy to outline the current status of the field. Now that the fundamental tools are outlined, it is time to start the exploration of how materials, molecules, and devices can control or utilize interactions with entangled photons.
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| Additional Information: | © 2020 The Royal Society of Chemistry. Submitted 13 May 2020; Accepted 19 May 2020; First published 19 May 2020. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-SC0020151. There are no conflicts to declare. | |||||||||
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| Issue or Number: | 31 | |||||||||
| Record Number: | CaltechAUTHORS:20200526-082511578 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20200526-082511578 | |||||||||
| Official Citation: | Entangled light-matter interactions and spectroscopy. J. Mater. Chem. C, 2020, 8, 10732-10741; doi: 10.1039/d0tc02300k | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 103436 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Tony Diaz | |||||||||
| Deposited On: | 26 May 2020 16:09 | |||||||||
| Last Modified: | 14 Aug 2020 16:59 |
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