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A continuous metal-insulator transition driven by spin correlations

Feng, Yejun and Wang, Yishu and Silevitch, D. M. and Cooper, S. E. and Mandrus, D. and Lee, Patrick A. and Rosenbaum, T. F. (2021) A continuous metal-insulator transition driven by spin correlations. Nature Communications, 12 . Art. No. 2779. ISSN 2041-1723. PMCID PMC8119431. doi:10.1038/s41467-021-23039-6. https://resolver.caltech.edu/CaltechAUTHORS:20201111-082624574

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Abstract

While Mott insulators induced by Coulomb interactions are a well-recognized class of metal-insulator transitions, insulators purely driven by spin correlations are much less common, as the reduced energy scale often invites competition from other degrees of freedom. Here, we demonstrate a clean example of a spin-correlation-driven metal-insulator transition in the all-in-all-out pyrochlore antiferromagnet Cd₂Os₂O₇, where the lattice symmetry is preserved by the antiferromagnetism. After the antisymmetric linear magnetoresistance from conductive, ferromagnetic domain walls is removed experimentally, the bulk Hall coefficient reveals four Fermi surfaces of both electron and hole types, sequentially departing the Fermi level with decreasing temperature below the Néel temperature, T_N = 227 K. In Cd₂Os₂O₇, the charge gap of a continuous metal-insulator transition opens only at T ~ 10 K << T_N. The insulating mechanism parallels the Slater picture, but without a folded Brillouin zone, and contrasts sharply with Mott insulators and spin density waves, where the electronic gap opens above and at T_N, respectively.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1038/s41467-021-23039-6DOIArticle
https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8119431PubMed CentralArticle
https://arxiv.org/abs/2009.13277arXivDiscussion Paper
ORCID:
AuthorORCID
Feng, Yejun0000-0003-3667-056X
Wang, Yishu0000-0002-5171-8376
Silevitch, D. M.0000-0002-6347-3513
Mandrus, D.0000-0003-3616-7104
Additional Information:© The Author(s) 2021. This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. Received 25 August 2020; Accepted 14 April 2021; Published 13 May 2021. Y.F. acknowledges support from the Okinawa Institute of Science and Technology Graduate University, with subsidy funding from the Cabinet Office, Government of Japan. The work at Caltech was supported by NSF DMR-Condensed Matter Physics. D.M.S. acknowledges support from AFOSR Grant No. FA9550-20-1-0263. P.A.L. acknowledges support from the US Department of Energy, Basic Energy Sciences, Grant No. DE-FG02-03ER46076. D.M. acknowledges support from the US Department of Energy, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering. Data availability: The data that support the findings of this study are available from the corresponding authors upon reasonable request. Author Contributions: Y.F., Y.W., P.A.L., and T.F.R. conceived of the research; D.M. provided the samples; Y.F., Y.W., D.M.S., and S.E.C. performed the experiments; Y.F., Y.W., P.A.L., and T.F.R. analyzed the data and prepared the manuscript. The authors declare no competing interests. Peer review information: Nature Communications thanks the anonymous reviewer(s) for their contribution to the peer review of this work.
Funders:
Funding AgencyGrant Number
Okinawa Institute of Science and TechnologyUNSPECIFIED
Cabinet Office (Japan)UNSPECIFIED
NSFDMR-1606858
Air Force Office of Scientific Research (AFOSR)FA9550-20-1-0263
Department of Energy (DOE)DE-FG02-03ER46076
Subject Keywords:Electronic properties and materials; Magnetic properties and materials; Phase transitions and critical phenomena
PubMed Central ID:PMC8119431
DOI:10.1038/s41467-021-23039-6
Record Number:CaltechAUTHORS:20201111-082624574
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20201111-082624574
Official Citation:Feng, Y., Wang, Y., Silevitch, D.M. et al. A continuous metal-insulator transition driven by spin correlations. Nat Commun 12, 2779 (2021). https://doi.org/10.1038/s41467-021-23039-6
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:106607
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:11 Nov 2020 16:47
Last Modified:17 May 2021 18:06

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