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Excitons in a reconstructed moiré potential in twisted WSe₂/WSe₂ homobilayers

Andersen, Trond I. and Scuri, Giovanni and Sushko, Andrey and De Greve, Kristiaan and Sung, Jiho and Zhou, You and Wild, Dominik S. and Gelly, Ryan J. and Heo, Hoseok and Bérubé, Damien and Joe, Andrew Y. and Jauregui, Luis A. and Watanabe, Kenji and Taniguchi, Takashi and Kim, Philip and Park, Hongkun and Lukin, Mikhail D. (2021) Excitons in a reconstructed moiré potential in twisted WSe₂/WSe₂ homobilayers. Nature Materials, 20 (4). pp. 480-487. ISSN 1476-1122. doi:10.1038/s41563-020-00873-5. https://resolver.caltech.edu/CaltechAUTHORS:20210112-080355149

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Abstract

Moiré superlattices in twisted van der Waals materials have recently emerged as a promising platform for engineering electronic and optical properties. A major obstacle to fully understanding these systems and harnessing their potential is the limited ability to correlate direct imaging of the moiré structure with optical and electronic properties. Here we develop a secondary electron microscope technique to directly image stacking domains in fully functional van der Waals heterostructure devices. After demonstrating the imaging of AB/BA and ABA/ABC domains in multilayer graphene, we employ this technique to investigate reconstructed moiré patterns in twisted WSe₂/WSe₂ bilayers and directly correlate the increasing moiré periodicity with the emergence of two distinct exciton species in photoluminescence measurements. These states can be tuned individually through electrostatic gating and feature different valley coherence properties. We attribute our observations to the formation of an array of two intralayer exciton species that reside in alternating locations in the superlattice, and open up new avenues to realize tunable exciton arrays in twisted van der Waals heterostructures, with applications in quantum optoelectronics and explorations of novel many-body systems.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1038/s41563-020-00873-5DOIArticle
https://rdcu.be/cdrNUPublisherFree ReadCube access
https://arxiv.org/abs/1912.06955arXivDiscussion Paper
ORCID:
AuthorORCID
Scuri, Giovanni0000-0003-1050-3114
Sung, Jiho0000-0002-7390-4567
Zhou, You0000-0002-9854-545X
Wild, Dominik S.0000-0001-7994-7077
Watanabe, Kenji0000-0003-3701-8119
Kim, Philip0000-0002-8255-0086
Park, Hongkun0000-0001-9576-8829
Lukin, Mikhail D.0000-0002-8658-1007
Alternate Title:Excitons in a reconstructed moiré potential in twisted WSe2/WSe2 homobilayers, Moiré Excitons Correlated with Superlattice Structure in Twisted WSe2/WSe2 Homobilayers, Moiré Excitons Correlated with Superlattice Structure in Twisted WSe₂/WSe₂ Homobilayers
Additional Information:© 2020 Nature Publishing Group. Received 12 February 2020; Accepted 11 November 2020; Published 04 January 2021. We thank B. Urbaszek, R. Bekenstein and L. Ju for helpful discussions. We acknowledge support from the DoD Vannevar Bush Faculty Fellowship (N00014-16-1-2825 for H.P. and N00014-18-1-2877 for P.K.), NSF (PHY-1506284 for H.P. and M.D.L.), NSF CUA (PHY-1125846 for H.P. and M.D.L.), AFOSR MURI (FA9550-17-1-0002) and ARL (W911NF1520067) for H.P. and M.D.L., the Gordon and Betty Moore Foundation (GBMF4543 for P.K.), ONR MURI (N00014-15-1-2761 for P.K.) and Samsung Electronics (for P.K. and H.P.). All the fabrication was performed at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Coordinated Infrastructure Network (NNCI), which is supported by the National Science Foundation under NSF award 1541959. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan, and the CREST (JPMJCR15F3), JST. A.S. acknowledges support from the Fannie and John Hertz Foundation and the Paul & Daisy Soros Fellowships for New Americans. Data availability: All data needed to evaluate the conclusions are presented in the article and the Supplementary Information. Author Contributions: T.I.A., G.S., A.S., K.D.G., H.P. and M.D.L. conceived the project. T.I.A., G.S., A.S. and K.D.G. designed and performed the experiments, analysed the data and wrote the manuscript with extensive input from the other authors. Y.Z. and J.S. assisted with the optical measurements. T.I.A., G.S., J.S., Y.Z., L.A.J. and A.Y.J. fabricated the samples. A.S. and K.D.G. performed the SEM imaging. T.I.A., G.S., A.S., K.D.G, D.S.W. and D.B. developed the theoretical model. H.H. grew the TMD crystals. T.T. and K.W. grew the hBN crystals. P.K., H.P. and M.D.L. supervised the project. The authors declare no competing interests.
Funders:
Funding AgencyGrant Number
Department of DefenseUNSPECIFIED
Office of Naval Research (ONR)N00014-16-1-2825
Office of Naval Research (ONR)N00014-18-1-2877
NSFPHY-1506284
NSFPHY-1125846
Air Force Office of Scientific Research (AFOSR)FA9550-17-1-0002
Army Research Office (ARO)W911NF1520067
Gordon and Betty Moore FoundationGBMF4543
Office of Naval Research (ONR)N00014-15-1-2761
Samsung ElectronicsUNSPECIFIED
NSFECCS-1541959
Ministry of Education, Culture, Sports, Science and Technology (MEXT)UNSPECIFIED
Japan Science and Technology AgencyJPMJCR15F3
Fannie and John Hertz FoundationUNSPECIFIED
Paul and Daisy Soros FellowshipUNSPECIFIED
Subject Keywords:Condensed-matter physics; Electronic devices; Electronic properties and materials; Semiconductors; Two-dimensional materials
Issue or Number:4
DOI:10.1038/s41563-020-00873-5
Record Number:CaltechAUTHORS:20210112-080355149
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20210112-080355149
Official Citation:Andersen, T.I., Scuri, G., Sushko, A. et al. Excitons in a reconstructed moiré potential in twisted WSe2/WSe2 homobilayers. Nat. Mater. 20, 480–487 (2021). https://doi.org/10.1038/s41563-020-00873-5
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:107412
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:12 Jan 2021 16:36
Last Modified:30 Mar 2021 19:33

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