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Simultaneous Reciprocal and Real Space X-Ray Imaging of Time-Evolving Systems

Kagias, Matias and Wang, Zhentian and Lovric, Goran and Jefimovs, Konstantins and Stampanoni, Marco (2021) Simultaneous Reciprocal and Real Space X-Ray Imaging of Time-Evolving Systems. Physical Review Applied, 15 (4). Art. No. 044038. ISSN 2331-7019. https://resolver.caltech.edu/CaltechAUTHORS:20210626-222733562

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Abstract

Imaging the (sub)micron scale over large areas with high temporal resolution becomes increasingly necessary for the development and investigation of novel materials under realistic operation conditions. Small angle x-ray scattering imaging methods provide micro- and nanoscale structural information of materials. A fundamental shortcoming of such methods is the long acquisition time required to investigate macroscopic objects. In this work, we propose a single shot imaging method that allows reciprocal space sensitivity at a local level while maintaining spatial resolution for imaging macroscopic objects. We use an instrument that is sensitive to the ultrasmall angle x-ray scattering range and utilize it to image unstable polydisperse particle systems. This allows us to observe in real time the evolution of the local average particle diameter due to the stratification of the microparticles.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1103/physrevapplied.15.044038DOIArticle
ORCID:
AuthorORCID
Kagias, Matias0000-0003-0435-6672
Wang, Zhentian0000-0002-1646-1405
Lovric, Goran0000-0002-0833-4043
Additional Information:© 2021 American Physical Society. (Received 23 November 2020; revised 12 February 2021; accepted 7 April 2021; published 23 April 2021) The imaging experiments were performed at the TOMCAT beamline of the Swiss Light Source, PSI Villigen, Switzerland. The fabrication of the optical elements was performed at the laboratory of micro and nanofabrication (LMN), PSI Villigen, Switzerland. Part of this work is funded by the Eurostars Grant E!1106 INFORMAT, SNF Sinergia Grant CRSII5_18356 “Clinical GI-BCT,” and the lottery fund SwissLOS of the Canton of Aargau.
Funders:
Funding AgencyGrant Number
EurostarsE!1106 INFORMAT
Swiss National Science Foundation (SNSF)CRSII5_18356
SwissLOS of the Canton of AargauUNSPECIFIED
Issue or Number:4
Record Number:CaltechAUTHORS:20210626-222733562
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20210626-222733562
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:109613
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:28 Jun 2021 18:17
Last Modified:28 Jun 2021 18:17

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