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New challenges in oxygen reduction catalysis: a consortium retrospective to inform future research

Burke Stevens, Michaela and Anand, Megha and Kreider, Melissa E. and Price, Eliza K. and Zamara Zeledón, José and Wang, Liang and Peng, Jiayu and Li, Hao and Gregoire, John M. and Hummelshøj, Jens and Jaramillo, Thomas F. and Jia, Hongfei and Nørskov, Jens K. and Roman-Leshkov, Yuriy and Shao-Horn, Yang and Storey, Brian D. and Suram, Santosh K. and Torrisi, Steven B. and Montoya, Joseph H. (2022) New challenges in oxygen reduction catalysis: a consortium retrospective to inform future research. Energy and Environmental Science, 15 (9). pp. 3775-3794. ISSN 1754-5692. doi:10.1039/d2ee01333a. https://resolver.caltech.edu/CaltechAUTHORS:20220811-235016000

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Abstract

In this perspective, we highlight results of a research consortium devoted to advancing understanding of oxygen reduction reaction (ORR) catalysis as a means to inform fuel cell science. We demonstrate how targeted collaborations between different institutions from academic, national lab, and industry backgrounds and different scientific disciplines like theory, experiment, and characterization can yield unique insights into fuel cell catalysts. We comment on such insights into material designs for platinum-group-metal alloys, transition metal oxides, and non-traditional materials including metal–organic frameworks; systems that have served as the foundational building blocks for our consortium. We also motivate a renewed focus on catalyst durability in light of emerging technological requirements and paths forward in understanding in situ and operando electrochemical stability. Finally, we describe new frontiers ORR research can take and how emerging artificial intelligence tools can assist researchers in capturing data, selecting new experiments, and guiding characterization to accelerate the design and discovery of fuel cell catalysts. A main goal of sharing this perspective is to discuss the rationale for our future research plans based on our consortium work. However, we also hope to illustrate both the potential impact of a collaborative strategy with the hopes of inspiring a higher degree of Industry-Academia-National Laboratory collaboration and encourage other centers and consortiums to distill and share their findings in a similar perspective-type article. Together we hope to enable the fuel cell research community to engage in a discussion of strategies for research and accelerated development of catalysts with improved activity and stability.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1039/D2EE01333ADOIArticle
ORCID:
AuthorORCID
Burke Stevens, Michaela0000-0003-3584-0600
Anand, Megha0000-0003-2707-3587
Kreider, Melissa E.0000-0003-1750-6860
Zamara Zeledón, José0000-0002-2205-0303
Peng, Jiayu0000-0003-3696-770X
Li, Hao0000-0002-7577-1366
Gregoire, John M.0000-0002-2863-5265
Jaramillo, Thomas F.0000-0001-9900-0622
Nørskov, Jens K.0000-0002-4427-7728
Roman-Leshkov, Yuriy0000-0002-0025-4233
Shao-Horn, Yang0000-0001-8714-2121
Storey, Brian D.0000-0001-5612-3390
Suram, Santosh K.0000-0001-8170-2685
Torrisi, Steven B.0000-0002-4283-8077
Montoya, Joseph H.0000-0001-5760-2860
Additional Information:© The Royal Society of Chemistry 2022. Received 24th April 2022, Accepted 12th July 2022. This work is supported by the Energy and Materials Division of the Toyota Research Institute. Author contributions. J. M. G., J. H., T. F. J., J. K. N., Y. R.-L., Y. S.-H., B. S., S. K. S., and J. H. M. conceived and outlined the perspective content. M. B. S., J. H. M., L. W. and H. J. wrote Section 1 and the Summary. M. B. S., M. A., M. E. K., E. K. P., H. L., J. P., J. Z. Z., and J. M. G. wrote Section 2. M. B. S., M. E. K., and J. H. M. wrote Section 3. J. H. M, S. B. T., and S. K. S. wrote Section 4. M. B. S. and J. H. M. organized and coordinated the writing and revision. All authors contributed to editing and manuscript revision. Conflicts of interest. J. H., S. S., S. B. T., and J. H. M., have patents pending and granted related to fuel cell and materials discovery technology.
Funders:
Funding AgencyGrant Number
Toyota Research InstituteUNSPECIFIED
Issue or Number:9
DOI:10.1039/d2ee01333a
Record Number:CaltechAUTHORS:20220811-235016000
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20220811-235016000
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:116255
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:12 Aug 2022 23:15
Last Modified:03 Dec 2022 02:01

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