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Challenges and opportunities in continuous flow processes for electrochemically mediated carbon capture

Liu, Yayuan and Lucas, Éowyn and Sullivan, Ian and Li, Xing and Xiang, Chengxiang (2022) Challenges and opportunities in continuous flow processes for electrochemically mediated carbon capture. iScience, 25 (10). Art. No. 105153. ISSN 2589-0042. PMCID PMC9529983. doi:10.1016/j.isci.2022.105153. https://resolver.caltech.edu/CaltechAUTHORS:20221208-575982500.9

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Abstract

Carbon capture from both stationary emitters and dilute sources is critically needed to mitigate climate change. Carbon dioxide separation methods driven by electrochemical stimuli show promise to sidestep the high-energy penalty and fossil-fuel dependency associated with the conventional pressure and temperature swings. Compared with a batch process, electrochemically mediated carbon capture (EMCC) operating in a continuous flow mode offers greater design flexibility. Therefore, this review introduces key advances in continuous flow EMCC for point source, air, and ocean carbon captures. Notably, the main challenges and future research opportunities for practical implementation of continuous flow EMCC processes are discussed from a multi-scale perspective, from molecules to electrochemical cells and finally to separation systems.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1016/j.isci.2022.105153DOIArticle
http://www.ncbi.nlm.nih.gov/pmc/articles/pmc9529983/PubMed CentralArticle
ORCID:
AuthorORCID
Lucas, Éowyn0000-0002-8743-5722
Sullivan, Ian0000-0003-0632-4607
Xiang, Chengxiang0000-0002-1698-6754
Additional Information:The authors would like to acknowledge funding from Johns Hopkins University and the Scialog program sponsored jointly by Research Corporation for Science Advancement and the Alfred P. Sloan Foundation, with additional support from Climate Pathfinders Foundation (grant #28438).
Funders:
Funding AgencyGrant Number
Johns Hopkins UniversityUNSPECIFIED
Scialog Fellow of Research CorporationUNSPECIFIED
Alfred P. Sloan FoundationUNSPECIFIED
Climate Pathfinders Foundation28438
Issue or Number:10
PubMed Central ID:PMC9529983
DOI:10.1016/j.isci.2022.105153
Record Number:CaltechAUTHORS:20221208-575982500.9
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20221208-575982500.9
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:118277
Collection:CaltechAUTHORS
Deposited By: Research Services Depository
Deposited On:11 Jan 2023 15:41
Last Modified:17 Jan 2023 18:45

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