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EELS femtosecond resolved in 4D ultrafast electron microscopy

Carbone, Fabrizio and Barwick, Brett and Kwon, Oh-Hoon and Park, Hyun Soon and Baskin, J. Spencer and Zewail, Ahmed H. (2009) EELS femtosecond resolved in 4D ultrafast electron microscopy. Chemical Physics Letters, 468 (4-6). pp. 107-111. ISSN 0009-2614. https://resolver.caltech.edu/CaltechAUTHORS:CARcpl09

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Abstract

Electron energy loss spectroscopy (EELS) is a powerful tool in the study of valency, bonding and structure of solids. Previously, EEL spectra were either time-integrated or at best time-resolved on the millisecond to seconds scale, being limited by video rates and detector responses. Here, using our 4D electron microscope, we report ultrafast EELS, taking the time resolution in the energy–time space into the femtosecond regime, a 10 order of magnitude increase, and for a table-top apparatus. It is shown that the energy–time–amplitude space of graphite is selective to changes, especially in the electron density of the π + σ plasmon of the collective oscillation of the four electrons of carbon.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1016/j.cplett.2008.12.027DOIArticle
http://www.sciencedirect.com/science/article/pii/S0009261408016552PublisherArticle
ORCID:
AuthorORCID
Kwon, Oh-Hoon0000-0001-7114-8617
Additional Information:© 2008 Elsevier. Received 25 November 2008; accepted 9 December 2008. Available online 16 December 2008. This work was supported by the National Science Foundation and the Air Force Office of Scientific Research in the Gordon and Betty Moore Center for Physical Biology at Caltech. The authors thank Profs. Marlina A. Elburg and Petra Rudolf for providing the raw crystals.
Funders:
Funding AgencyGrant Number
NSFUNSPECIFIED
Air Force Office of Scientific Research (AFOSR)UNSPECIFIED
Gordon and Betty Moore FoundationUNSPECIFIED
Issue or Number:4-6
Record Number:CaltechAUTHORS:CARcpl09
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:CARcpl09
Official Citation:Fabrizio Carbone, Brett Barwick, Oh-Hoon Kwon, Hyun Soon Park, J. Spencer Baskin, Ahmed H. Zewail, EELS femtosecond resolved in 4D ultrafast electron microscopy, Chemical Physics Letters, Volume 468, Issues 4–6, 22 January 2009, Pages 107-111, ISSN 0009-2614, http://dx.doi.org/10.1016/j.cplett.2008.12.027. (http://www.sciencedirect.com/science/article/pii/S0009261408016552)
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ID Code:13206
Collection:CaltechAUTHORS
Deposited By: Archive Administrator
Deposited On:02 Feb 2009 23:41
Last Modified:09 Mar 2020 13:18

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