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Long-range pollution transport during the MILAGRO-2006 campaign: a case study of a major Mexico City outflow event using free-floating altitude-controlled balloons

Voss, P. B. and Zaveri, R. A. and Flocke, F. M. and Mao, H. and Hartley, T. P. and DeAmicis, P. and Deonandan, I. and Contreras-Jiménez, G. and Martínez-Antonio, O. and Figueroa Estrada, M. and Greenberg, D. and Campos, T. L. and Weinheimer, A. J. and Knapp, D. J. and Montzka, D. D. and Crounse, J. D. and Wennberg, P. O. and Apel, E. and Madronich, S. and de Foy, B. (2010) Long-range pollution transport during the MILAGRO-2006 campaign: a case study of a major Mexico City outflow event using free-floating altitude-controlled balloons. Atmospheric Chemistry and Physics, 10 (15). pp. 7137-7159. ISSN 1680-7316. https://resolver.caltech.edu/CaltechAUTHORS:20100915-094034098

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Abstract

One of the major objectives of the Megacities Initiative: Local And Global Research Observations (MILAGRO-2006) campaign was to investigate the long-range transport of polluted Mexico City Metropolitan Area (MCMA) outflow and determine its downwind impacts on air quality and climate. Six research aircraft, including the National Center for Atmospheric Research (NCAR) C-130, made extensive chemical, aerosol, and radiation measurements above MCMA and more than 1000 km downwind in order to characterize the evolution of the outflow as it aged and dispersed over the Mesa Alta, Sierra Madre Oriental, Coastal Plain, and Gulf of Mexico. As part of this effort, free-floating Controlled-Meteorological (CMET) balloons, commanded to change altitude via satellite, made repeated profile measurements of winds and state variables within the advecting outflow. In this paper, we present an analysis of the data from two CMET balloons that were launched near Mexico City on the afternoon of 18 March 2006 and floated downwind with the MCMA pollution for nearly 30 h. The repeating profile measurements show the evolving structure of the outflow in considerable detail: its stability and stratification, interaction with other air masses, mixing episodes, and dispersion into the regional background. Air parcel trajectories, computed directly from the balloon wind profiles, show three transport pathways on 18–19 March: (a) high-altitude advection of the top of the MCMA mixed layer, (b) mid-level outflow over the Sierra Madre Oriental followed by decoupling and isolated transport over the Gulf of Mexico, and (c) low-level outflow with entrainment into a cleaner northwesterly jet above the Coastal Plain. The C-130 aircraft intercepted the balloon-based trajectories three times on 19 March, once along each of these pathways; in all three cases, peaks in urban tracer concentrations and LIDAR backscatter are consistent with MCMA pollution. In comparison with the transport models used in the campaign, the balloon-based trajectories appear to shear the outflow far more uniformly and decouple it from the surface, thus forming a thin but expansive polluted layer over the Gulf of Mexico that is well aligned with the aircraft observations. These results provide critical context for the extensive aircraft measurements made during the 18–19 March MCMA outflow event and may have broader implications for modelling and understanding long-range transport.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.5194/acp-10-7137-2010DOIArticle
http://www.atmos-chem-phys.net/10/7137/2010/PublisherArticle
ORCID:
AuthorORCID
Crounse, J. D.0000-0001-5443-729X
Wennberg, P. O.0000-0002-6126-3854
Additional Information:© Author(s) 2010. This work is distributed under the Creative Commons Attribution 3.0 License. Received: 22 January 2010; Published in Atmos. Chem. Phys. Discuss.: 9 February 2010. Revised: 28 June 2010; Accepted: 16 July 2010; Published: 4 August 2010. We gratefully acknowledge the support of the National Science Foundation Atmospheric Chemistry Program (Grant Numbers: ATM-0511833, ATM-0810950, and ATM- 0511803), the National Center for Atmospheric Research (NCAR), the Servicios a la Navegacíon en el Espacio Aéreo Mexicano (SENEAM), Instituto Nacional de Ecología (INE), pilots and crew of the C-130, José Meitín at NCAR, Sandra I. Ramírez Jiménez at the Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, and our many gracious hosts in Mexico. The C-130 meteorological data and SABL imagery was provided by NCAR/EOL under sponsorship of the National Science Foundation. All analysis was performed in the Matlab (v7.0.1) programming environment from the MathWorks Inc. Edited by: L. Molina.
Funders:
Funding AgencyGrant Number
NSFATM-0511833
NSFATM-0810950
NSFATM- 0511803
National Center for Atmospheric Research (NCAR)UNSPECIFIED
Servicios a la Navegación en el Espacio Aéreo Mexicano (SENEAM)UNSPECIFIED
Instituto Nacional de Ecología (INE)UNSPECIFIED
Universidad Nacional Autónoma de México (UNAM)UNSPECIFIED
Issue or Number:15
Record Number:CaltechAUTHORS:20100915-094034098
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20100915-094034098
Official Citation:Voss, P. B., Zaveri, R. A., Flocke, F. M., Mao, H., Hartley, T. P., DeAmicis, P., Deonandan, I., Contreras-Jiménez, G., Martínez-Antonio, O., Figueroa Estrada, M., Greenberg, D., Campos, T. L., Weinheimer, A. J., Knapp, D. J., Montzka, D. D., Crounse, J. D., Wennberg, P. O., Apel, E., Madronich, S., and de Foy, B.: Long-range pollution transport during the MILAGRO-2006 campaign: a case study of a major Mexico City outflow event using free-floating altitude-controlled balloons, Atmos. Chem. Phys., 10, 7137-7159, doi:10.5194/acp-10-7137-2010, 2010.
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:19967
Collection:CaltechAUTHORS
Deposited By: Jason Perez
Deposited On:15 Sep 2010 18:17
Last Modified:03 Oct 2019 02:03

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