Grain Aggregate Experiments NO PRIOR RELEASE 25% PRIOR RELEEASE Ea Ea 0 Kcal s-1 Prior Release Fo Kcal s-1 Prior Release Fo Grain A 33 800000 0 Grain A 32.9676 800000 0.249915205 Grain B 33 1600000 Grain B 32.9676 1600000 CA/CB 1 CA/CB 1 Release Coordinate Fi 3He Fi 4He Release Coordinate Fi 3He Fi 4He y=y1=y3 Aggregate y=y1=y3 Aggregate Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) 1 0.000001 0.000002 0.004096 0.005790 0.004096 0.005790 0.999997 -21.131366 1 0.000001 0.000002 0.004096 0.005790 0.000026 0.000052 0.010556 -21.131366 2 0.000003 0.000005 0.003072 0.004338 0.003072 0.004338 1.000000 -20.408163 2 0.000003 0.000005 0.003072 0.004338 0.000054 0.000108 0.029112 -20.408163 3 0.000006 0.000012 0.003816 0.005384 0.003816 0.005384 1.000000 -19.714894 3 0.000006 0.000012 0.003816 0.005384 0.000108 0.000216 0.047051 -19.714894 4 0.000013 0.000025 0.004997 0.007043 0.004997 0.007043 1.000000 -19.050474 4 0.000013 0.000025 0.004997 0.007043 0.000211 0.000422 0.070125 -19.050474 5 0.000025 0.000051 0.006611 0.009304 0.006611 0.009304 1.000000 -18.413777 5 0.000025 0.000051 0.006611 0.009304 0.000401 0.000800 0.100671 -18.413777 6 0.000049 0.000098 0.008721 0.012249 0.008721 0.012249 1.000000 -17.803863 6 0.000049 0.000098 0.008721 0.012249 0.000743 0.001477 0.141159 -17.803863 7 0.000092 0.000184 0.011410 0.015985 0.011410 0.015985 1.000000 -17.183990 7 0.000092 0.000184 0.011410 0.015985 0.001341 0.002651 0.194280 -17.183990 8 0.000168 0.000336 0.014775 0.020627 0.014775 0.020627 1.000000 -16.612705 8 0.000168 0.000336 0.014775 0.020627 0.002357 0.004619 0.262707 -16.612705 9 0.000300 0.000601 0.018914 0.026285 0.018914 0.026285 1.000000 -16.062846 9 0.000300 0.000601 0.018914 0.026285 0.004031 0.007783 0.348459 -16.062846 10 0.000526 0.001052 0.023921 0.033045 0.023921 0.033045 1.000000 -15.533478 10 0.000526 0.001052 0.023921 0.033045 0.006688 0.012617 0.451799 -15.533478 11 0.000903 0.001807 0.029872 0.040943 0.029872 0.040943 1.000000 -15.023776 11 0.000903 0.001807 0.029872 0.040943 0.010717 0.019553 0.569906 -15.023776 12 0.001523 0.003047 0.036806 0.049933 0.036806 0.049933 1.000000 -14.533019 12 0.001523 0.003047 0.036806 0.049933 0.016501 0.028790 0.696148 -14.533019 13 0.002526 0.005052 0.044704 0.059843 0.044704 0.059843 1.000000 -14.060586 13 0.002526 0.005052 0.044704 0.059843 0.024272 0.040110 0.821035 -14.060586 14 0.004121 0.008241 0.053458 0.070319 0.053458 0.070319 1.000000 -13.605942 14 0.004121 0.008241 0.053458 0.070319 0.033966 0.052836 0.934958 -13.605942 15 0.006619 0.013238 0.062831 0.080759 0.062831 0.080759 1.000000 -13.168612 15 0.006619 0.013238 0.062831 0.080759 0.045142 0.065917 1.031178 -13.168612 16 0.010478 0.020956 0.072413 0.090245 0.072413 0.090245 1.000000 -12.748101 16 0.010478 0.020956 0.072413 0.090245 0.057034 0.078049 1.107204 -12.748101 17 0.016357 0.032714 0.081566 0.097480 0.081566 0.097480 1.000000 -12.343695 17 0.016357 0.032714 0.081566 0.097480 0.068641 0.087698 1.164144 -12.343695 18 0.025196 0.050392 0.089382 0.100765 0.089382 0.100765 1.000000 -11.953884 18 0.025196 0.050392 0.089382 0.100765 0.078793 0.093008 1.204595 -11.953884 19 0.038321 0.076642 0.094643 0.095692 0.094643 0.095692 1.000000 -11.589590 19 0.038321 0.076642 0.094643 0.095692 0.086136 0.089332 1.229088 -11.589590 20 0.057580 0.115159 0.095464 0.080350 0.095464 0.080350 1.000000 -11.249923 20 0.057580 0.115159 0.095464 0.080350 0.088428 0.075610 1.243928 -11.249923 21 0.085518 0.171035 0.087946 0.054934 0.087946 0.054934 1.000000 -10.943751 21 0.085518 0.171035 0.087946 0.054934 0.082473 0.051848 1.253357 -10.943751 22 0.125608 0.251215 0.071272 0.027699 0.071272 0.027699 1.000000 -10.676735 22 0.125608 0.251215 0.071272 0.027699 0.067132 0.026155 1.256654 -10.676735 23 8.074382 16.148764 0.079310 0.010989 0.079310 0.010989 1.000000 -9.016830 23 8.074382 16.148764 0.079310 0.010989 0.074890 0.010383 1.259033 -9.016830 Ea Ea 0.000000 Kcal s-1 Prior Release Fo Kcal s-1 Prior Release Fo Grain A 32.967600 800000.000000 0.000000 Grain A 32.967600 800000.000000 0.249915 Grain B 32.967600 1600000.000000 Grain B 32.967600 1600000.000000 CA/CB 0.333330 CA/CB 0.333330 Release Coordinate Fi 3He Fi 4He Release Coordinate Fi 3He Fi 4He y=y1=y3 Aggregate y=y1=y3 Aggregate Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) 1 0.000001 0.000002 0.004096 0.005790 0.004096 0.005790 0.914334 -21.131366 1 0.000001 0.000002 0.004096 0.005790 0.000026 0.000052 0.008797 -21.131366 2 0.000003 0.000005 0.003072 0.004338 0.003072 0.004338 0.914553 -20.408163 2 0.000003 0.000005 0.003072 0.004338 0.000054 0.000108 0.024263 -20.408163 3 0.000006 0.000012 0.003816 0.005384 0.003816 0.005384 0.914762 -19.714894 3 0.000006 0.000012 0.003816 0.005384 0.000108 0.000216 0.039218 -19.714894 4 0.000013 0.000025 0.004997 0.007043 0.004997 0.007043 0.915032 -19.050474 4 0.000013 0.000025 0.004997 0.007043 0.000211 0.000422 0.058464 -19.050474 5 0.000025 0.000051 0.006611 0.009304 0.006611 0.009304 0.915390 -18.413777 5 0.000025 0.000051 0.006611 0.009304 0.000401 0.000800 0.083966 -18.413777 6 0.000049 0.000098 0.008721 0.012249 0.008721 0.012249 0.915868 -17.803863 6 0.000049 0.000098 0.008721 0.012249 0.000743 0.001477 0.117826 -17.803863 7 0.000092 0.000184 0.011410 0.015985 0.011410 0.015985 0.916504 -17.183990 7 0.000092 0.000184 0.011410 0.015985 0.001341 0.002651 0.162392 -17.183990 8 0.000168 0.000336 0.014775 0.020627 0.014775 0.020627 0.917348 -16.612705 8 0.000168 0.000336 0.014775 0.020627 0.002357 0.004619 0.220115 -16.612705 9 0.000300 0.000601 0.018914 0.026285 0.018914 0.026285 0.918460 -16.062846 9 0.000300 0.000601 0.018914 0.026285 0.004031 0.007783 0.293123 -16.062846 10 0.000526 0.001052 0.023921 0.033045 0.023921 0.033045 0.919920 -15.533478 10 0.000526 0.001052 0.023921 0.033045 0.006688 0.012617 0.382407 -15.533478 11 0.000903 0.001807 0.029872 0.040943 0.029872 0.040943 0.921830 -15.023776 11 0.000903 0.001807 0.029872 0.040943 0.010717 0.019553 0.486722 -15.023776 12 0.001523 0.003047 0.036806 0.049933 0.036806 0.049933 0.924328 -14.533019 12 0.001523 0.003047 0.036806 0.049933 0.016501 0.028790 0.601697 -14.533019 13 0.002526 0.005052 0.044704 0.059843 0.044704 0.059843 0.927596 -14.060586 13 0.002526 0.005052 0.044704 0.059843 0.024272 0.040110 0.720034 -14.060586 14 0.004121 0.008241 0.053458 0.070319 0.053458 0.070319 0.931890 -13.605942 14 0.004121 0.008241 0.053458 0.070319 0.033966 0.052836 0.833314 -13.605942 15 0.006619 0.013238 0.062831 0.080759 0.062831 0.080759 0.937573 -13.168612 15 0.006619 0.013238 0.062831 0.080759 0.045142 0.065917 0.934715 -13.168612 16 0.010478 0.020956 0.072413 0.090245 0.072413 0.090245 0.945185 -12.748101 16 0.010478 0.020956 0.072413 0.090245 0.057034 0.078049 1.021060 -12.748101 17 0.016357 0.032714 0.081566 0.097480 0.081566 0.097480 0.955561 -12.343695 17 0.016357 0.032714 0.081566 0.097480 0.068641 0.087698 1.093172 -12.343695 18 0.025196 0.050392 0.089382 0.100765 0.089382 0.100765 0.970069 -11.953884 18 0.025196 0.050392 0.089382 0.100765 0.078793 0.093008 1.154739 -11.953884 19 0.038321 0.076642 0.094643 0.095692 0.094643 0.095692 0.997244 -11.589590 19 0.038321 0.076642 0.094643 0.095692 0.086136 0.089332 1.217876 -11.589590 20 0.057580 0.115159 0.095464 0.080350 0.095464 0.080350 1.042985 -11.249923 20 0.057580 0.115159 0.095464 0.080350 0.088428 0.075610 1.292507 -11.249923 21 0.085518 0.171035 0.087946 0.054934 0.087946 0.054934 1.115524 -10.943751 21 0.085518 0.171035 0.087946 0.054934 0.082473 0.051848 1.396217 -10.943751 22 0.125608 0.251215 0.071272 0.027699 0.071272 0.027699 1.220129 -10.676735 22 0.125608 0.251215 0.071272 0.027699 0.067132 0.026155 1.532626 -10.676735 23 8.074382 16.148764 0.079310 0.010989 0.079310 0.010989 1.378310 -9.016830 23 8.074382 16.148764 0.079310 0.010989 0.074890 0.010383 1.735220 -9.016830 Ea Ea 0.000000 Kcal s-1 Prior Release Fo Kcal s-1 Prior Release Fo Grain A 32.967600 800000.000000 0.000000 Grain A 32.967600 800000.000000 0.249915 Grain B 32.967600 1600000.000000 Grain B 32.967600 1600000.000000 CA/CB 3.000000 CA/CB 3.000000 Release Coordinate Fi 3He Fi 4He Release Coordinate Fi 3He Fi 4He y=y1=y3 Aggregate y=y1=y3 Aggregate Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) Step Grain a Grain b Grain a Grain b Grain a Grain b 4He/3He ln(D3He) 1 0.000001 0.000002 0.004096 0.005790 0.004096 0.005790 1.085660 -21.131366 1 0.000001 0.000002 0.004096 0.005790 0.000026 0.000052 0.012314 -21.131366 2 0.000003 0.000005 0.003072 0.004338 0.003072 0.004338 1.085446 -20.408163 2 0.000003 0.000005 0.003072 0.004338 0.000054 0.000108 0.033962 -20.408163 3 0.000006 0.000012 0.003816 0.005384 0.003816 0.005384 1.085237 -19.714894 3 0.000006 0.000012 0.003816 0.005384 0.000108 0.000216 0.054884 -19.714894 4 0.000013 0.000025 0.004997 0.007043 0.004997 0.007043 1.084967 -19.050474 4 0.000013 0.000025 0.004997 0.007043 0.000211 0.000422 0.081786 -19.050474 5 0.000025 0.000051 0.006611 0.009304 0.006611 0.009304 1.084609 -18.413777 5 0.000025 0.000051 0.006611 0.009304 0.000401 0.000800 0.117377 -18.413777 6 0.000049 0.000098 0.008721 0.012249 0.008721 0.012249 1.084131 -17.803863 6 0.000049 0.000098 0.008721 0.012249 0.000743 0.001477 0.164492 -17.803863 7 0.000092 0.000184 0.011410 0.015985 0.011410 0.015985 1.083495 -17.183990 7 0.000092 0.000184 0.011410 0.015985 0.001341 0.002651 0.226169 -17.183990 8 0.000168 0.000336 0.014775 0.020627 0.014775 0.020627 1.082652 -16.612705 8 0.000168 0.000336 0.014775 0.020627 0.002357 0.004619 0.305301 -16.612705 9 0.000300 0.000601 0.018914 0.026285 0.018914 0.026285 1.081539 -16.062846 9 0.000300 0.000601 0.018914 0.026285 0.004031 0.007783 0.403798 -16.062846 10 0.000526 0.001052 0.023921 0.033045 0.023921 0.033045 1.080080 -15.533478 10 0.000526 0.001052 0.023921 0.033045 0.006688 0.012617 0.521193 -15.533478 11 0.000903 0.001807 0.029872 0.040943 0.029872 0.040943 1.078169 -15.023776 11 0.000903 0.001807 0.029872 0.040943 0.010717 0.019553 0.653092 -15.023776 12 0.001523 0.003047 0.036806 0.049933 0.036806 0.049933 1.075672 -14.533019 12 0.001523 0.003047 0.036806 0.049933 0.016501 0.028790 0.790601 -14.533019 13 0.002526 0.005052 0.044704 0.059843 0.044704 0.059843 1.072403 -14.060586 13 0.002526 0.005052 0.044704 0.059843 0.024272 0.040110 0.922038 -14.060586 14 0.004121 0.008241 0.053458 0.070319 0.053458 0.070319 1.068109 -13.605942 14 0.004121 0.008241 0.053458 0.070319 0.033966 0.052836 1.036604 -13.605942 15 0.006619 0.013238 0.062831 0.080759 0.062831 0.080759 1.062426 -13.168612 15 0.006619 0.013238 0.062831 0.080759 0.045142 0.065917 1.127644 -13.168612 16 0.010478 0.020956 0.072413 0.090245 0.072413 0.090245 1.054815 -12.748101 16 0.010478 0.020956 0.072413 0.090245 0.057034 0.078049 1.193350 -12.748101 17 0.016357 0.032714 0.081566 0.097480 0.081566 0.097480 1.044439 -12.343695 17 0.016357 0.032714 0.081566 0.097480 0.068641 0.087698 1.235118 -12.343695 18 0.025196 0.050392 0.089382 0.100765 0.089382 0.100765 1.029931 -11.953884 18 0.025196 0.050392 0.089382 0.100765 0.078793 0.093008 1.254453 -11.953884 19 0.038321 0.076642 0.094643 0.095692 0.094643 0.095692 1.002756 -11.589590 19 0.038321 0.076642 0.094643 0.095692 0.086136 0.089332 1.240302 -11.589590 20 0.057580 0.115159 0.095464 0.080350 0.095464 0.080350 0.957016 -11.249923 20 0.057580 0.115159 0.095464 0.080350 0.088428 0.075610 1.195348 -11.249923 21 0.085518 0.171035 0.087946 0.054934 0.087946 0.054934 0.884477 -10.943751 21 0.085518 0.171035 0.087946 0.054934 0.082473 0.051848 1.110494 -10.943751 22 0.125608 0.251215 0.071272 0.027699 0.071272 0.027699 0.779873 -10.676735 22 0.125608 0.251215 0.071272 0.027699 0.067132 0.026155 0.980674 -10.676735 23 8.074382 16.148764 0.079310 0.010989 0.079310 0.010989 0.621692 -9.016830 23 8.074382 16.148764 0.079310 0.010989 0.074890 0.010383 0.782835 -9.016830 Diffusion Experiment -1 Ea 0.000000 Kcal s-1 Grain A 32.967600 800000.000000 Grain B 32.967600 1600000.000000 CA/CB 1.000000 Release Coordinate Fi 3He y=y1=y3 Step Grain a Grain b Grain a Grain b ln(D3He) 1 0.000002 0.000003 0.005790 0.011559 -20.699625 2 0.000005 0.000010 0.002461 0.004902 -19.977879 3 0.000012 0.000024 0.003466 0.006890 -19.285264 4 0.000025 0.000051 0.004774 0.009466 -18.622148 5 0.000051 0.000102 0.006462 0.012771 -17.987457 6 0.000098 0.000196 0.008619 0.016953 -17.380395 7 0.000184 0.000368 0.011339 0.022162 -16.755397 8 0.000336 0.000672 0.014725 0.028538 -16.186239 9 0.000601 0.001202 0.018878 0.036182 -15.639204 10 0.001052 0.002104 0.023895 0.045128 -15.113567 11 0.001807 0.003613 0.029853 0.055296 -14.608779 12 0.003047 0.006094 0.036791 0.066432 -14.124498 13 0.005052 0.010104 0.044693 0.078023 -13.660624 14 0.008241 0.016482 0.053450 0.089215 -13.217370 15 0.013238 0.026476 0.062825 0.098713 -12.795360 16 0.020956 0.041912 0.072408 0.104714 -12.395783 17 0.032714 0.065427 0.081563 0.103830 -12.027500 18 0.050392 0.100783 0.089379 0.091467 -11.709342 19 0.076642 0.153284 0.094640 0.066562 -11.455022 20 0.115159 0.230318 0.095462 0.035958 -11.248331 21 0.171035 0.342070 0.087945 0.012589 -11.054637 22 0.251215 0.502430 0.071271 0.002435 -10.800226 23 16.148764 32.297528 0.079309 0.000215 -9.049760 Diffusion Experiment -2 Release Coordinate Fi 3He y=y1=y3 Step Grain a Grain b Grain a ln(D3He) 1 0.000002 0.000003 0.257369 -12.307217 2 0.000005 0.000010 0.130702 -11.955474 3 0.000012 0.000024 0.119244 -11.628497 4 0.000025 0.000051 0.115116 -11.369704 5 0.000051 0.000102 0.110559 -11.180776 6 0.000098 0.000196 0.099330 -11.014626 7 0.000184 0.000368 0.079587 -10.786631 Diffusion Experiment -3 Release Coordinate Fi 3He y=y1=y3 Step Grain a Grain b Grain a ln(D3He) 1 0.000002 0.000003 0.004096 -20.697930 2 0.000005 0.000010 0.003072 -19.975890 3 0.000012 0.000024 0.003816 -19.283943 4 0.000025 0.000051 0.004997 -18.621234 5 0.000051 0.000102 0.006611 -17.986810 6 0.000098 0.000196 0.008721 -17.379928 7 0.000184 0.000368 0.011410 -16.755324 8 0.000336 0.000672 0.014775 -16.186184 9 0.000601 0.001202 0.018914 -15.639163 10 0.001052 0.002104 0.023921 -15.113536 11 0.001807 0.003613 0.029872 -14.608755 12 0.003047 0.006094 0.036806 -14.124479 13 0.005052 0.010104 0.044704 -13.660609 14 0.008241 0.016482 0.053458 -13.217358 15 0.013238 0.026476 0.062831 -12.795350 16 0.020956 0.041912 0.072413 -12.395775 17 0.032714 0.065427 0.081566 -12.027490 18 0.050392 0.100783 0.089382 -11.709331 19 0.076642 0.153284 0.094643 -11.455011 20 0.115159 0.230318 0.095464 -11.248323 21 0.171035 0.342070 0.087946 -11.054633 22 0.251215 0.502430 0.071272 -10.800225