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Geophysical applications of nuclear resonant spectroscopy

Sturhahn, Wolfgang and Jackson, Jennifer M. (2007) Geophysical applications of nuclear resonant spectroscopy. In: Advances in High-Pressure Mineralogy. Geological Society of America Special Papers. No.421. Geological Society of America , Boulder, CO, pp. 157-174. ISBN 9780813724218. https://resolver.caltech.edu/CaltechAUTHORS:20130109-144406768

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Abstract

We summarize recent developments of nuclear resonant spectroscopy methods, such as nuclear resonant inelastic X-ray scattering and synchrotron Mössbauer spectroscopy, and their uses for the geophysical sciences. The inelastic method provides specific vibrational information, for example, the phonon density of states, and, in combination with compression data, it permits the determination of sound velocities and Grüneisen parameters under high pressure and high temperature. The Mössbauer method provides hyperfine interactions between the resonant nucleus and electronic environment, such as isomer shifts, quadrupole splittings, and magnetic fields, which provide important information on valence, spin state, and magnetic ordering. Both methods use a nuclear resonant isotope as a probe and can be applied under high pressure and high temperature. The physical mechanism of nuclear resonant scattering and the specifics in applications to Earth materials are presented with reference to several high-pressure studies on iron-bearing compounds.


Item Type:Book Section
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1130/2007.2421(09)DOIUNSPECIFIED
http://specialpapers.gsapubs.org/content/421/157PublisherUNSPECIFIED
ORCID:
AuthorORCID
Sturhahn, Wolfgang0000-0002-9606-4740
Jackson, Jennifer M.0000-0002-8256-6336
Additional Information:© 2007 Geological Society of America. Manuscript Accepted by the Society 14 August 2006. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357.
Group:Seismological Laboratory
Funders:
Funding AgencyGrant Number
Department of Energy (DOE) Office of Science, Office of Basic Energy SciencesDE-AC02-06CH11357
Subject Keywords:phonon density of states, sound velocities, Gruneisen parameter, magnetism, nuclear resonant scattering
Series Name:Geological Society of America Special Papers
Issue or Number:421
Record Number:CaltechAUTHORS:20130109-144406768
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20130109-144406768
Official Citation:Sturhahn, W., and Jackson, J.M., 2007, Geophysical applications of nuclear resonant spectroscopy, in Ohtani, E., ed., Advances in High-Pressure Mineralogy: Geological Society of America Special Paper 421, p. 157-174, doi: 10.1130/2007.2421(09)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:36281
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:14 Jan 2013 22:59
Last Modified:24 Jan 2020 18:04

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