CaltechAUTHORS
  A Caltech Library Service

Measurements of methane emissions at natural gas production sites in the United States

Allen, David T. and Torres, Vincent M. and Thomas, James and Sullivan, David W. and Harrison, Matthew and Hendler, Al and Herndon, Scott C. and Kolb, Charles E. and Fraser, Matthew P. and Hill, A. Daniel and Lamb, Brian K. and Miskimins, Jennifer and Sawyer, Robert F. and Seinfeld, John H. (2013) Measurements of methane emissions at natural gas production sites in the United States. Proceedings of the National Academy of Sciences of the United States of America, 110 (44). pp. 17768-17773. ISSN 0027-8424. PMCID PMC3816463. https://resolver.caltech.edu/CaltechAUTHORS:20131210-101910500

[img]
Preview
PDF - Published Version
See Usage Policy.

956Kb
[img]
Preview
PDF - Supplemental Material
See Usage Policy.

2357Kb

Use this Persistent URL to link to this item: https://resolver.caltech.edu/CaltechAUTHORS:20131210-101910500

Abstract

Engineering estimates of methane emissions from natural gas production have led to varied projections of national emissions. This work reports direct measurements of methane emissions at 190 onshore natural gas sites in the United States (150 production sites, 27 well completion flowbacks, 9 well unloadings, and 4 workovers). For well completion flowbacks, which clear fractured wells of liquid to allow gas production, methane emissions ranged from 0.01 Mg to 17 Mg (mean = 1.7 Mg; 95% confidence bounds of 0.67–3.3 Mg), compared with an average of 81 Mg per event in the 2011 EPA national emission inventory from April 2013. Emission factors for pneumatic pumps and controllers as well as equipment leaks were both comparable to and higher than estimates in the national inventory. Overall, if emission factors from this work for completion flowbacks, equipment leaks, and pneumatic pumps and controllers are assumed to be representative of national populations and are used to estimate national emissions, total annual emissions from these source categories are calculated to be 957 Gg of methane (with sampling and measurement uncertainties estimated at ±200 Gg). The estimate for comparable source categories in the EPA national inventory is ∼1,200 Gg. Additional measurements of unloadings and workovers are needed to produce national emission estimates for these source categories. The 957 Gg in emissions for completion flowbacks, pneumatics, and equipment leaks, coupled with EPA national inventory estimates for other categories, leads to an estimated 2,300 Gg of methane emissions from natural gas production (0.42% of gross gas production).


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1073/pnas.1304880110DOIArticle
http://www.pnas.org/content/110/44/17768PublisherArticle
http://www.pnas.org/content/110/44/17768/suppl/DCSupplementalPublisherSupporting Information
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3816463/PubMed CentralArticle
ORCID:
AuthorORCID
Seinfeld, John H.0000-0003-1344-4068
Additional Information:© 2013 National Academy of Sciences. Freely available online through the PNAS open access option. Edited by Susan L. Brantley, Pennsylvania State University, University Park, PA, and approved August 19, 2013 (received for review March 20, 2013). We thank the sponsors of this work for financial support, technical advice, and access to sites for sampling. The sponsors were Environmental Defense Fund (EDF), Anadarko Petroleum Corporation, BG Group plc, Chevron, Encana Oil & Gas (USA) Inc., Pioneer Natural Resources Company, SWEPI LP (Shell), Southwestern Energy, Talisman Energy USA, and XTO Energy, an ExxonMobil subsidiary. Funding for EDF’s methane research series, including the University of Texas study, is provided for by Fiona and Stan Druckenmiller, Heising-Simons Foundation, Bill and Susan Oberndorf, Betsy and Sam Reeves, Robertson Foundation, Tom Steyer, Kat Taylor, and the Walton Family Foundation. Author contributions: D.T.A. and M.H. designed research; D.T.A., V.M.T., J.T., D.W.S., M.H., A.H., and S.C.H. performed research; C.E.K., M.P.F., A.D.H., B.K.L., J.M., R.F.S., and J.H.S. analyzed data; and D.T.A. wrote the paper. Conflict of interest statement: J.M. holds a joint appointment with Barree & Associates and the Colorado School of Mines. She has also served as an advisor to Nexen in 2012. D.T.A. served as a consultant for the Eastern Research Group and ExxonMobil in 2012, and is the current chair of the Science Advisory Board for the EPA. J.H.S. has served as a consultant for Shell in 2012. D.T.A., M.H., C.E.K., and R.F.S. variously serve as members of scientific advisory panels for projects supported by Environmental Defense Fund and companies involved in the natural gas supply chain. These projects are led at Colorado State University (on natural gas gathering and processing), Washington State University (on local distribution of natural gas), and the University of West Virginia (on CNG fueling and use in heavy duty vehicles). This article is a PNAS Direct Submission. This article contains supporting information online at www.pnas.org/lookup/suppl/doi:10.1073/pnas.1304880110/-/DCSupplemental.
Funders:
Funding AgencyGrant Number
Environmental Defense FundUNSPECIFIED
Anadarko Petroleum CorporationUNSPECIFIED
BG Group plcUNSPECIFIED
ChevronUNSPECIFIED
Encana Oil & Gas (USA) Inc.UNSPECIFIED
Pioneer Natural Resources CompanyUNSPECIFIED
SWEPI LP (Shell)UNSPECIFIED
Southwestern EnergyUNSPECIFIED
Talisman Energy USAUNSPECIFIED
XTO EnergyUNSPECIFIED
Exxon MobilUNSPECIFIED
Fiona and Stan DruckenmillerUNSPECIFIED
Heising-Simons FoundationUNSPECIFIED
Bill and Susan ObernorfUNSPECIFIED
Betsy and Sam ReevesUNSPECIFIED
Robertson FoundationUNSPECIFIED
Tom SteyerUNSPECIFIED
Kat TaylorUNSPECIFIED
Walton Family Foundation UNSPECIFIED
Subject Keywords:greenhouse gas emissions, hydraulic fracturing
Issue or Number:44
PubMed Central ID:PMC3816463
Record Number:CaltechAUTHORS:20131210-101910500
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20131210-101910500
Official Citation:David T. Allen, Vincent M. Torres, James Thomas, David W. Sullivan, Matthew Harrison, Al Hendler, Scott C. Herndon, Charles E. Kolb, Matthew P. Fraser, A. Daniel Hill, Brian K. Lamb, Jennifer Miskimins, Robert F. Sawyer, and John H. Seinfeld Measurements of methane emissions at natural gas production sites in the United States PNAS 2013 110 (44) 17768-17773; published ahead of print September 16, 2013, doi:10.1073/pnas.1304880110
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:42919
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:10 Dec 2013 19:28
Last Modified:03 Oct 2019 06:03

Repository Staff Only: item control page