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Global distribution and climate forcing of carbonaceous aerosols

Chung, Serena H. and Seinfeld, John H. (2002) Global distribution and climate forcing of carbonaceous aerosols. Journal of Geophysical Research D, 107 (D19). Art. No. 4407. ISSN 0148-0227. doi:10.1029/2001JD001397. https://resolver.caltech.edu/CaltechAUTHORS:20141027-100415884

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Abstract

The global distribution of carbonaceous aerosols is simulated online in the Goddard Institute for Space Studies General Circulation Model II-prime (GISS GCM II-prime). Prognostic tracers include black carbon (BC), primary organic aerosol (POA), five groups of biogenic volatile organic compounds (BVOCs), and 14 semivolatile products of BVOC oxidation by O_3, OH, and NO_3, which condense to form secondary organic aerosols (SOA) based on an equilibrium partitioning model and experimental observations. Estimated global burdens of BC, organic carbon (OC), and SOA are 0.22, 1.2, and 0.19 Tg with lifetimes of 6.4, 5.3, and 6.2 days, respectively. The predicted global production of SOA is 11.2 Tg yr^(−1), with 91% due to O_3 and OH oxidation. Globally averaged, top of the atmosphere (TOA) radiative forcing by anthropogenic BC is predicted as +0.51 to +0.8 W m^(−2), the former being for BC in an external mixture and the latter for BC in an internal mixture of sulfate, OC, and BC. Globally averaged, anthropogenic BC, OC, and sulfate are predicted to exert a TOA radiative forcing of −0.39 to −0.78 W m^(−2), depending on the exact assumptions of aerosol mixing and water uptake by OC. Forcing estimates are compared with those published previously.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1029/2001JD001397DOIArticle
http://onlinelibrary.wiley.com/doi/10.1029/2001JD001397/abstractPublisherArticle
ORCID:
AuthorORCID
Seinfeld, John H.0000-0003-1344-4068
Additional Information:Copyright 2002 by the American Geophysical Union. Received 15 October 2001; revised 12 April 2002; accepted 13 June 2002; published 15 October 2002. This work was supported by the National Aeronautics and Space Administration Earth Observing System Interdisciplinary Science Program (NASA EOS-IDS). Serena Chung was supported by a National Science Foundation Graduate Fellowship. The authors thank Peter Adams and Dorothy Koch for assistance.
Funders:
Funding AgencyGrant Number
NASAUNSPECIFIED
NSF Graduate Research FellowshipUNSPECIFIED
Issue or Number:D19
Classification Code:0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0360 Atmospheric Composition and Structure: Transmission and scattering of radiation; 0365 Atmospheric Composition and Structure: Troposphere—composition and chemistry
DOI:10.1029/2001JD001397
Record Number:CaltechAUTHORS:20141027-100415884
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20141027-100415884
Official Citation:Chung, S. H., and J. H. Seinfeld, Global distribution and climate forcing of carbonaceous aerosols, J. Geophys. Res., 107(D19), 4407, doi:10.1029/2001JD001397, 2002.
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:50836
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:27 Oct 2014 17:21
Last Modified:10 Nov 2021 19:01

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