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A comparison of scavenging and deposition processes in global models: results from the WCRP Cambridge Workshop of 1995

Rasch, P. J. and Seinfeld, J. (2000) A comparison of scavenging and deposition processes in global models: results from the WCRP Cambridge Workshop of 1995. Tellus B, 52 (4). pp. 1025-1056. ISSN 0280-6509. http://resolver.caltech.edu/CaltechAUTHORS:20141103-133304101

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Abstract

We report on results from a World Climate Research Program workshop on representations of scavenging and deposition processes in global transport models of the atmosphere. 15 models were evaluated by comparing simulations of radon, lead, sulfur dioxide, and sulfate against each other, and against observations of these constituents. This paper provides a survey on the simulation differences between models. It identifies circumstances where models are consistent with observations or with each other, and where they differ from observations or with each other. The comparison shows that most models are able to simulate seasonal species concentrations near the surface over continental sites to within a factor of 2 over many regions of the globe. Models tend to agree more closely over source (continental) regions than for remote (polar and oceanic) regions. Model simulations differ most strongly in the upper troposphere for species undergoing wet scavenging processes. There are not a sufficient number of observations to characterize the climatology (long-term average) of species undergoing wet scavenging in the upper troposphere. This highlights the need for either a different strategy for model evaluation (e.g., comparisons on an event by event basis) or many more observations of a few carefully chosen constituents.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1034/j.1600-0889.2000.00980.xDOIArticle
http://www.tellusb.net/index.php/tellusb/article/view/17091PublisherArticle
ORCID:
AuthorORCID
Seinfeld, J.0000-0003-1344-4068
Additional Information:Copyright © Munksgaard, 2000. This journal is published under the terms of the Creative Commons Attribution 4.0 International (CC-BY 4.0) License. (Manuscript received 17 November 1998; in final form 15 December 1999). We would like to thank the World Climate Research Programme and V. Savtchenko for funding the workshop. We thank Richard Larsen, G. Polian, and members of the EMEFS science teams for providing their data to us prior to its publication. We thank Daniel Jacob and Brian Eaton for comments on the first draft of the manuscript and Henning Rodhe and an anonymous referee for their comments during the review process. Work at the Met Office was supported by the UK Department of Environment, Transport and the Regions under contract PECD/7/12/37.
Funders:
Funding AgencyGrant Number
World Climate Research ProgrammeUNSPECIFIED
Department of Environment, Transport and the Regions (UK)PECD/7/12/37
Record Number:CaltechAUTHORS:20141103-133304101
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20141103-133304101
Official Citation:RASCH, P. J., FEICHTER, J., LAW, K., MAHOWALD, N., PENNER, J., BENKOVITZ, C., GENTHON, C., GIANNAKOPOULOS, C., KASIBHATLA, P., KOCH, D., LEVY, H., MAKI, T., PRATHER, M., ROBERTS, D. L., ROELOFS, G.-J., STEVENSON, D., STOCKWELL, Z., TAGUCHI, S., KRITZ, M., CHIPPERFIELD, M., BALDOCCHI, D., McMURRY, P., BARRIE, L., BALKANSKI, Y., CHATFIELD, R., KJELLSTROM, E., LAWRENCE, M., LEE, H. N., LELIEVELD, J., NOONE, K. J., SEINFELD, J., STENCHIKOV, G., SCHWARTZ, S., WALCEK, C. and WILLIAMSON, D. (2000), A comparison of scavenging and deposition processes in global models: results from the WCRP Cambridge Workshop of 1995. Tellus B, 52: 1025–1056. doi: 10.1034/j.1600-0889.2000.00980.x
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:51183
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:03 Nov 2014 21:57
Last Modified:20 Sep 2017 21:14

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