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Semiconductor Surface Transformations for Photoelectrochemical Energy Conversion

Lewerenz, Hans J. (2014) Semiconductor Surface Transformations for Photoelectrochemical Energy Conversion. Journal of the Electrochemical Society, 161 (13). H3117-H3129. ISSN 0013-4651. https://resolver.caltech.edu/CaltechAUTHORS:20150108-085815861

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Abstract

The issue of photoelectrode stability, while simultaneously maintaining efficient operation in aqueous solutions, is addressed for energy converting half cells and complete photoelectrocatalytic structures. The historical development of stability concepts, their realization and recent advances are described. Examples are presented that span the time from the inception of photoelectrochemical energy conversion to present day's renewed interest in storable solar energy. The application of (photo)corrosion processes for in-situ synthesis of protective coatings is described and chemical and electronic analyses of the interphases formed are given. Future development and innovation routes will be discussed.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1149/2.0211413jes DOIArticle
http://jes.ecsdl.org/content/161/13/H3117PublisherArticle
ORCID:
AuthorORCID
Lewerenz, Hans J.0000-0001-8433-9471
Alternate Title:JES Focus Issue in Recognition of Adam Heller and His Enduring Contributions to Electrochemistry
Additional Information:© 2014 The Electrochemical Society. Manuscript submitted October 6, 2014; revised manuscript received November 10, 2014. Published December 3, 2014. This paper is part of the JES Focus Issue in Recognition of Adam Heller and His Enduring Contributions to Electrochemistry. The author is indebted to the Bell Laboratories team led by Adam Heller, which also included Barry Miller, Klaus Bachmann, Shalini Menezes, Ferdinand Thiel and Dave Aspnes; from the group at the Hahn-Meitner Institute in Berlin (now the Helmholtz Zentrum Berlin after merging with the synchrotron facility Bessy II), I acknowledge contributions of Mohammed Aggour, Juergen Grzanna, Thomas Stempel, Andres Munoz, Katarzyna Skorupska Christian Heine, Thomas Hannappel, Matthias May, Oliver Supplie and Ulrike Bloeck. At Caltech, enlightening discussions with Matthew Shaner, Katherine Fountaine and Harry Atwater are gratefully acknowledged. Part of the work described here was funded by the DFG (Project No. LE 1192–4). This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, as follows: the composition and the writing of the review as well as the modeling results were supported through the Office of Science of the US Department of Energy under Award No. DE-SC00049993.
Group:JCAP
Funders:
Funding AgencyGrant Number
Deutsche Forschungsgemeinschaft (DFG)LE 1192-4
Department of Energy (DOE)DE-SC00049993
Issue or Number:13
Record Number:CaltechAUTHORS:20150108-085815861
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20150108-085815861
Official Citation:Hans J. Lewerenz Semiconductor Surface Transformations for Photoelectrochemical Energy Conversion J. Electrochem. Soc. 2014 161(13): H3117-H3129; doi:10.1149/2.0211413jes
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:53328
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:09 Jan 2015 19:39
Last Modified:08 Oct 2019 22:02

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