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Highly ordered nanowire arrays on plastic substrates for ultrasensitive flexible chemical sensors

McAlpine, Michael C. and Ahmad, Habib and Wang, Dunwei and Heath, James R. (2007) Highly ordered nanowire arrays on plastic substrates for ultrasensitive flexible chemical sensors. Nature Materials, 6 (5). pp. 379-384. ISSN 1476-1122. PMCID PMC3695594. https://resolver.caltech.edu/CaltechAUTHORS:20150317-125849636

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Abstract

The development of a robust method for integrating high-performance semiconductors on flexible plastics could enable exciting avenues in fundamental research and novel applications. One area of vital relevance is chemical and biological sensing, which if implemented on biocompatible substrates, could yield breakthroughs in implantable or wearable monitoring systems. Semiconducting nanowires (and nanotubes) are particularly sensitive chemical sensors because of their high surface-to-volume ratios. Here, we present a scalable and parallel process for transferring hundreds of pre-aligned silicon nanowires onto plastic to yield highly ordered films for low-power sensor chips. The nanowires are excellent field-effect transistors, and, as sensors, exhibit parts-per-billion sensitivity to NO_2, a hazardous pollutant. We also use SiO_2 surface chemistries to construct a 'nano-electronic nose' library, which can distinguish acetone and hexane vapours via distributed responses. The excellent sensing performance coupled with bendable plastic could open up opportunities in portable, wearable or even implantable sensors.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1038/nmat1891DOIArticle
https://rdcu.be/clgPPublisherFree ReadCube access
https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3695594PubMed CentralArticle
ORCID:
AuthorORCID
Heath, James R.0000-0001-5356-4385
Additional Information:© 2007 Nature Publishing Group. Received 12 January 2007; accepted 21 March 2007; published 22 April 2007. We thank W. Dichtel, A. Boukai and Y. Bunimovich for useful discussions. M.C.M. thanks the Intelligence Community Postdoctoral Research Fellowship Program for financial support. J.R.H. acknowledges primary support of this work via a contract from the MITRE Corporation, and support from the National Cancer Institute (#5U54 CA119347). Author contributions: M.C.M. and J.R.H. conceived the experiments, M.C.M. carried out the experiments and M.C.M., H.A. and D.W. designed the experiments.
Funders:
Funding AgencyGrant Number
Intelligence Community Postdoctoral Research FellowshipUNSPECIFIED
MITRE CorporationUNSPECIFIED
National Cancer Institute5U54 CA119347
Issue or Number:5
PubMed Central ID:PMC3695594
Record Number:CaltechAUTHORS:20150317-125849636
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20150317-125849636
Official Citation:McAlpine, M., Ahmad, H., Wang, D. et al. Highly ordered nanowire arrays on plastic substrates for ultrasensitive flexible chemical sensors. Nature Mater 6, 379–384 (2007) doi:10.1038/nmat1891
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:55857
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:17 Mar 2015 21:46
Last Modified:23 Dec 2019 16:44

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