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Semiclassical Dressed State Theory for the Vibrational Excitation of a Morse Oscillator by Radiation

Voth, Gregory A. and Marcus, R. A. (1985) Semiclassical Dressed State Theory for the Vibrational Excitation of a Morse Oscillator by Radiation. Journal of Physical Chemistry, 89 (11). pp. 2208-2213. ISSN 0022-3654 . http://resolver.caltech.edu/CaltechAUTHORS:20150629-101153293

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Abstract

A uniform semiclassical theory is developed to treat the interaction of a Morse oscillator with a monochromatic radiation field. The correspondence with quantum-mechanical dressed state theory for the Rabi and resonant excitation frequencies is demonstrated, and the semiclassical theory is used to describe resonant one- and two-photon absorption processes. The results are extended to state-to-state vibrational excitation in a polyatomic species.


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http://dx.doi.org/10.1021/j100257a015DOIArticle
http://pubs.acs.org/doi/abs/10.1021/j100257a015PublisherArticle
Additional Information:© 1985 American Chemical Society. Received: September 28, 1984. This work has been supported by a grant from the National Science Foundation.
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Caltech Arthur Amos Noyes Laboratory of Chemical Physics7104
Record Number:CaltechAUTHORS:20150629-101153293
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20150629-101153293
Official Citation:Semiclassical dressed state theory for the vibrational excitation of a Morse oscillator by radiation Gregory A. Voth and R. A. Marcus The Journal of Physical Chemistry 1985 89 (11), 2208-2213
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:58660
Collection:CaltechAUTHORS
Deposited By: Jason Perez
Deposited On:29 Jun 2015 20:00
Last Modified:29 Jun 2015 20:01

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