A Caltech Library Service

In situ aerosol-size distributions and clear-column radiative closure during ACE-2

Collins, D. R. and Jonsson, H. H. and Seinfeld, J. H. and Flagan, R. C. and Gassó, S. and Hegg, D. A. and Russell, P. B. and Schmid, B. and Livingston, J. M. and Öström, E. and Noone, K. J. and Russell, L. M. and Putaud, J. P. (2000) In situ aerosol-size distributions and clear-column radiative closure during ACE-2. Tellus B, 52 (2). pp. 498-525. ISSN 0280-6509. doi:10.1034/j.1600-0889.2000.00008.x.

[img] PDF - Published Version
Creative Commons Attribution.


Use this Persistent URL to link to this item:


As part of the second Aerosol Characterization Experiment (ACE-2) during June and July of 1997, aerosol-size distributions were measured on board the CIRPAS Pelican aircraft through the use of a DMA and 2 OPCs. During the campaign, the boundary-layer aerosol typically possessed characteristics representative of a background marine aerosol or a continentally influenced aerosol, while the free-tropospheric aerosol was characterized by the presence or absence of a Saharan dust layer. A range of radiative closure comparisons were made using the data obtained during vertical profiles flown on 4 missions. Of particular interest here are the comparisons made between the optical properties as determined through the use of measured aerosol-size distributions and those measured directly by an airborne 14-wavelength sunphotometer and 3 nephelometers. Variations in the relative humidity associated with each of the direct measurements required consideration of the hygroscopic properties of the aerosol for size-distribution-based calculations. Simultaneous comparison with such a wide range of directly-measured optical parameters not only offers evidence of the validity of the physicochemical description of the aerosol when closure is achieved, but also provides insight into potential sources of error when some or all of the comparisons result in disagreement. Agreement between the derived and directly-measured optical properties varied for different measurements and for different cases. Averaged over the 4 case studies, the derived extinction coefficient at 525 nm exceeded that measured by the sunphotometer by 2.5% in the clean boundary layer, but underestimated measurements by 13% during pollution events. For measurements within the free troposphere, the mean derived extinction coefficient was 3.3% and 17% less than that measured by the sunphotometer during dusty and non-dusty conditions, respectively. Likewise, averaged discrepancies between the derived and measured scattering coefficient were −9.6%, +4.7%, +17%, and −41% for measurements within the clean boundary layer, polluted boundary layer, free troposphere with a dust layer, and free troposphere without a dust layer, respectively. Each of these quantities, as well as the majority of the >100 individual comparisons from which they were averaged, were within estimated uncertainties.

Item Type:Article
Related URLs:
URLURL TypeDescription
Jonsson, H. H.0000-0003-3043-1074
Seinfeld, J. H.0000-0003-1344-4068
Flagan, R. C.0000-0001-5690-770X
Russell, L. M.0000-0002-6108-2375
Additional Information:This journal is published under the terms of the Creative Commons Attribution 4.0 International (CC-BY 4.0) License. This is a contribution to the International Global Atmospheric Chemistry (IGAC) core project of the International Geosphere-Biosphere Programme (IGBP) and is part of the IGAC Aerosol Characterization Experiments (ACE). Primary funding for this work has been provided by the National Science Foundation Grant ATM-9614105, and by the Office of Naval Research Grant N00014-91-0119. Additional funding has been provided by the Office of Naval Research Grant N00014-97-1-0132, the National Aeronautics and Space Administration, the National Oceanic and Atmospheric Administration, and the European Commission DG XII.
Funding AgencyGrant Number
Office of Naval Research (ONR)N00014-91-0119
Office of Naval Research (ONR)N00014-97-1-0132
National Oceanic and Atmospheric Administration (NOAA)UNSPECIFIED
European Commission DG XIIUNSPECIFIED
Issue or Number:2
Record Number:CaltechAUTHORS:20150806-170600160
Persistent URL:
Official Citation:COLLINS, D. R. et al. In situ aerosol-size distributions and clear-column radiative closure during ACE-2. Tellus B, [S.l.], v. 52, n. 2, Dec. 2011. ISSN 1600-0889. Available at: <>. Date accessed: 07 Aug. 2015. doi:
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:59293
Deposited By: Irina Meininger
Deposited On:08 Aug 2015 03:12
Last Modified:10 Nov 2021 22:18

Repository Staff Only: item control page