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Probing wavepacket dynamics with femtosecond energy- and angle-resolved photoelectron spectroscopy

Arasaki, Yasuki and Takatsuka, Kazuo and Wang, Kwanghsi and McKoy, Vincent (2000) Probing wavepacket dynamics with femtosecond energy- and angle-resolved photoelectron spectroscopy. Journal of Electron Spectroscopy and Related Phenomena, 108 (1-3). pp. 89-98. ISSN 0368-2048. http://resolver.caltech.edu/CaltechAUTHORS:20151027-154129956

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Abstract

Femtosecond energy- and angle-resolved pump-probe photoelectron spectra of wavepackets in a double-minimum state of Na_2 are studied. These studies illustrate that a robust description of the photoionization dynamics significantly enhances the utility of time-resolved photoelectron spectroscopy as a probe of wavepackets and of the evolution of electronic structure, particularly in regions of avoided crossings, and that the dependence of these angular distributions on the relative polarizations of the pump and probe lasers can be exploited to monitor molecular alignment.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1016/S0368-2048(00)00148-1DOIArticle
http://www.sciencedirect.com/science/article/pii/S0368204800001481PublisherArticle
Additional Information:© 2000 Elsevier. The authors thank the Ministry of Education, Science, and Culture of Japan for sponsorship of their collaboration. This work was supported by a grant from the National Science Foundation.
Funders:
Funding AgencyGrant Number
Ministry of Education, Culture, Sports, Science and Technology (MEXT)UNSPECIFIED
NSFUNSPECIFIED
Subject Keywords:Femtosecond wavepacket; Photoelectron spectra; Photoelectron matrix element
Record Number:CaltechAUTHORS:20151027-154129956
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20151027-154129956
Official Citation:Yasuki Arasaki, Kazuo Takatsuka, Kwanghsi Wang, Vincent McKoy, Probing wavepacket dynamics with femtosecond energy- and angle-resolved photoelectron spectroscopy, Journal of Electron Spectroscopy and Related Phenomena, Volume 108, Issues 1–3, July 2000, Pages 89-98, ISSN 0368-2048, http://dx.doi.org/10.1016/S0368-2048(00)00148-1. (http://www.sciencedirect.com/science/article/pii/S0368204800001481)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:61609
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:28 Oct 2015 15:31
Last Modified:28 Oct 2015 16:37

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