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Energy- and angle-resolved pump–probe femtosecond photoelectron spectroscopy: Molecular rotation

Arasaki, Yasuki and Takatsuka, Kazuo and Wang, Kwanghsi and McKoy, Vincent (2001) Energy- and angle-resolved pump–probe femtosecond photoelectron spectroscopy: Molecular rotation. Journal of Chemical Physics, 114 (18). pp. 7941-7950. ISSN 0021-9606. https://resolver.caltech.edu/CaltechAUTHORS:20151110-101709607

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Abstract

We have incorporated a classical treatment of molecular rotation into our formulation of energy- and angle-resolved pump–probe photoelectron spectroscopy. This classical treatment provides a useful approach to extracting the photoelectron signal primarily associated with vibrational dynamics in cases where rotational motion is slow and the coupling between rotational and vibrational motion is weak. We illustrate its applicability with pump–probe photoelectron spectra for wave packets on the ^1Σ^+_u double-minimum state of Na_2.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1063/1.1361067DOIArticle
http://scitation.aip.org/content/aip/journal/jcp/114/18/10.1063/1.1361067PublisherArticle
Additional Information:© 2001 American Institute of Physics. (Received 6 December 2000; accepted 13 February 2001) This work has been supported by a grants from the Ministry of Education, Science, and Culture (Japan) and the National Science Foundation (U.S.).
Funders:
Funding AgencyGrant Number
Ministry of Education, Culture, Sports, Science and Technology (MEXT)UNSPECIFIED
NSFUNSPECIFIED
Issue or Number:18
Record Number:CaltechAUTHORS:20151110-101709607
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20151110-101709607
Official Citation:Energy- and angle-resolved pump–probe femtosecond photoelectron spectroscopy: Molecular rotation Arasaki, Yasuki and Takatsuka, Kazuo and Wang, Kwanghsi and McKoy, Vincent, The Journal of Chemical Physics, 114, 7941-7950 (2001), DOI:http://dx.doi.org/10.1063/1.1361067
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:62022
Collection:CaltechAUTHORS
Deposited By: George Porter
Deposited On:10 Nov 2015 21:13
Last Modified:03 Oct 2019 09:14

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