Arasaki, Yasuki and Takatsuka, Kazuo and Wang, Kwanghsi and McKoy, Vincent (2001) Energy- and angle-resolved pump–probe femtosecond photoelectron spectroscopy: Molecular rotation. Journal of Chemical Physics, 114 (18). pp. 7941-7950. ISSN 0021-9606. doi:10.1063/1.1361067. https://resolver.caltech.edu/CaltechAUTHORS:20151110-101709607
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Abstract
We have incorporated a classical treatment of molecular rotation into our formulation of energy- and angle-resolved pump–probe photoelectron spectroscopy. This classical treatment provides a useful approach to extracting the photoelectron signal primarily associated with vibrational dynamics in cases where rotational motion is slow and the coupling between rotational and vibrational motion is weak. We illustrate its applicability with pump–probe photoelectron spectra for wave packets on the ^1Σ^+_u double-minimum state of Na_2.
| Item Type: | Article | |||||||||
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| Additional Information: | © 2001 American Institute of Physics. (Received 6 December 2000; accepted 13 February 2001) This work has been supported by a grants from the Ministry of Education, Science, and Culture (Japan) and the National Science Foundation (U.S.). | |||||||||
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| Issue or Number: | 18 | |||||||||
| DOI: | 10.1063/1.1361067 | |||||||||
| Record Number: | CaltechAUTHORS:20151110-101709607 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20151110-101709607 | |||||||||
| Official Citation: | Energy- and angle-resolved pump–probe femtosecond photoelectron spectroscopy: Molecular rotation Arasaki, Yasuki and Takatsuka, Kazuo and Wang, Kwanghsi and McKoy, Vincent, The Journal of Chemical Physics, 114, 7941-7950 (2001), DOI:http://dx.doi.org/10.1063/1.1361067 | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 62022 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | George Porter | |||||||||
| Deposited On: | 10 Nov 2015 21:13 | |||||||||
| Last Modified: | 10 Nov 2021 22:56 |
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