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Molecular Steps of Neutral Sulfuric Acid and Dimethylamine Nucleation in CLOUD

Jokinen, Tuija and Sarnela, Nina and Sipilä, Mikko and Junninen, Heikki and Lehtipalo, Katrianne and Duplissy, Jonathan (2013) Molecular Steps of Neutral Sulfuric Acid and Dimethylamine Nucleation in CLOUD. In: Nucleation and Atmospheric Aerosols. AIP Conference Proceedings. No.1527. American Institute of Physics , Melville, NY, pp. 302-305. ISBN 978-0-7354-1152-4.

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We have run a set of experiments in the CLOUD chamber at CERN, Switzerland, studying the effect of dimethylamine (DMA) on sulfuric acid (SA)-water nucleation using a nitrate based Chemical Ionization Atmospheric Pressure ionization Time-Of-Flight Mass Spectrometer (CI-APi-TOF). Experiment was designed to produce neutral high m/z SA-DMA clusters in close to atmospherically relevant conditions to be detected and characterized by the CI-APi-TOF. We aimed in filling up the gap in measurement techniques from molecular level up to climatically relevant aerosol particles and thus improve our understanding of the role of sulfuric acid and DMA in atmospheric nucleation.

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Additional Information:© 2013 AIP Publishing LLC. Published online 24 May 2013. We would like to thank CERN for supporting CLOUD with important technical and financial resources, and for providing a particle beam from the CERN Proton Synchrotron. This research has received funding from the EC Seventh Framework Programme (Marie Curie Initial Training Network "CLOUD-ITN" no. 215072, MCITN "CLOUD-TRAIN" no. 316662, and ERC-Advanced "ATMNUCLE" grant no.227463), the German Federal Ministry of Education and Research (project nos. 01LK0902A and 01LK1222A), the Swiss National Science Foundation (project nos.200020_135307 and 206620_130527), the Academy of Finland (Center of Excellence project no. 1118615), the Academy of Finland (135054, 133872, 251427, c, 139995, 137749, 141217, 141451), the Finnish Funding Agency for Technology and Innovation, the Nessling Foundation, the Austrian Science Fund (FWF; project no. P19546 and L593), the Portuguese Foundation for Science and Technology (project no. CERN/FP/116387/2010), the Swedish Research Council, Vetenskapsrådet (grant 2011-5120), the Presidium of the Russian Academy of Sciences and Russian Foundation for Basic Research (grants 08-02-91006-CERN and 12-02-91522-CERN), the U.S. National Science Foundation (grants AGS1136479 and CHE1012293) and Pegasos (400798).
Funding AgencyGrant Number
Marie Curie Fellowship215072
Marie Curie Fellowship316662
European Research Council (ERC)227463
Bundesministerium für Bildung und Forschung (BMBF)01LK0902A
Bundesministerium für Bildung und Forschung (BMBF)01LK1222A
Swiss National Science Foundation (SNSF)200020_135307
Swiss National Science Foundation (SNSF)206620_130527
Academy of Finland1118615
Academy of Finland135054
Academy of Finland133872
Academy of Finland251427
Academy of Finland139995
Academy of Finland137749
Academy of Finland141217
Academy of Finland141451
Finnish Funding Agency for Technology and InnovationUNSPECIFIED
Nessling FoundationUNSPECIFIED
FWF Der WissenschaftsfondsP19546
FWF Der WissenschaftsfondsL593
Fundação para a Ciência e a Tecnologia (FCT)CERN/FP/116387/2010
Swedish Research CouncilUNSPECIFIED
Russian Academy of SciencesUNSPECIFIED
Russian Foundation for Basic Research08-02-91006-CERN
Russian Foundation for Basic Research12-02-91522-CERN
Subject Keywords:Sulfuric Acid, Mass Spectrometry, Chemical Ionization, Nucleation
Classification Code:PACS: 64.60.Q-, 82.80.Rt, 36.40.-c, 82.33.Tb, 92.60.Mt
Record Number:CaltechAUTHORS:20160422-092011813
Persistent URL:
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:66398
Deposited By: Ruth Sustaita
Deposited On:22 Apr 2016 16:42
Last Modified:22 Apr 2016 16:42

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