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Source apportionment of airborne particulate matter using organic compounds as tracers

Schauer, James J. and Rogge, Wolfgang F. and Hildemann, Lynn M. and Mazurek, Monica A. and Cass, Glen R. and Simoneit, Bernd R. T. (1996) Source apportionment of airborne particulate matter using organic compounds as tracers. Atmospheric Environment, 30 (22). pp. 3837-3855. ISSN 1352-2310 . http://resolver.caltech.edu/CaltechAUTHORS:20160628-134703173

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Abstract

A chemical mass balance receptor model based on organic compounds has been developed that relates sours; contributions to airborne fine particle mass concentrations. Source contributions to the concentrations of specific organic compounds are revealed as well. The model is applied to four air quality monitoring sites in southern California using atmospheric organic compound concentration data and source test data collected specifically for the purpose of testing this model. The contributions of up to nine primary particle source types can be separately identified in ambient samples based on this method, and approximately 85% of the organic fine aerosol is assigned to primary sources on an annual average basis. The model provides information on source contributions to fine mass concentrations, fine organic aerosol concentrations and individual organic compound concentrations. The largest primary source contributors to fine particle mass concentrations in Los Angeles are found to include diesel engine exhaust, paved road dust, gasoline-powered vehicle exhaust, plus emissions from food cooking and wood smoke, with smaller contribution:; from tire dust, plant fragments, natural gas combustion aerosol, and cigarette smoke. Once these primary aerosol source contributions are added to the secondary sulfates, nitrates and organics present, virtually all of the annual average fine particle mass at Los Angeles area monitoring sites can be assigned to its source.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1016/1352-2310(96)00085-4 DOIArticle
http://www.sciencedirect.com/science/article/pii/1352231096000854PublisherArticle
Additional Information:© 1996 Elsevier Science Ltd. First received 29 June 1995 and in final form 8 February 1996. Available online 24 February 1999. This research was supported by the Caltech Center for Air Quality Analysis. Acquisition of the source profile and ambient organic compound data was supported by the U. S. Environmental Protection Agency under agreement R-81377-01-0, by the California Air Resources Board under agreement A932-127, and by the South Coast Air Quality Management District.
Funders:
Funding AgencyGrant Number
Caltech Center for Air Quality AnalysisUNSPECIFIED
Environmental Protection Agency (EPA)R-81377-01-0
California Air Resources BoardA932-127
South Coast Air Quality Management District (SCAQMD)UNSPECIFIED
Subject Keywords:Receptor models, organic aerosol, fine particles, source contributions, emissions
Record Number:CaltechAUTHORS:20160628-134703173
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20160628-134703173
Official Citation:James J. Schauer, Wolfgang F. Rogge, Lynn M. Hildemann, Monica A. Mazurek, Glen R. Cass, Bernd R.T. Simoneit, Source apportionment of airborne particulate matter using organic compounds as tracers, Atmospheric Environment, Volume 30, Issue 22, November 1996, Pages 3837-3855, ISSN 1352-2310, http://dx.doi.org/10.1016/1352-2310(96)00085-4. (http://www.sciencedirect.com/science/article/pii/1352231096000854)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:68715
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:29 Jun 2016 15:44
Last Modified:29 Jun 2016 15:44

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