Xiang, Chengxiang and Weber, Adam Z. and Ardo, Shane and Berger, Alan and Chen, Yikai and Coridan, Robert and Fountaine, Katherine T. and Haussener, Sophia and Hu, Shu and Liu, Rui and Lewis, Nathan S. and Modestino, Miguel A. and Shaner, Matthew M. and Singh, Meenesh R. and Stevens, John C. and Sun, Ke and Walczak, Karl (2016) Modeling, Simulation, and Implementation of Solar-Driven Water-Splitting Devices. Angewandte Chemie International Edition, 55 (42). pp. 12974-12988. ISSN 1433-7851. doi:10.1002/anie.201510463. https://resolver.caltech.edu/CaltechAUTHORS:20160729-070531307
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Abstract
An integrated cell for the solar-driven splitting of water consists of multiple functional components and couples various photoelectrochemical (PEC) processes at different length and time scales. The overall solar-to-hydrogen (STH) conversion efficiency of such a system depends on the performance and materials properties of the individual components as well as on the component integration, overall device architecture, and system operating conditions. This Review focuses on the modeling- and simulation-guided development and implementation of solar-driven water-splitting prototypes from a holistic viewpoint that explores the various interplays between the components. The underlying physics and interactions at the cell level is are reviewed and discussed, followed by an overview of the use of the cell model to provide target properties of materials and guide the design of a range of traditional and unique device architectures.
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| Additional Information: | © 2016 Wiley-VCH Verlag GmbH & Co. Received: November 11, 2015. Revised: January 31, 2016. Version of Record online: 27 Jul 2016. We would like to thank the community of researchers whose work is reflected in this Review, especially those past and present at JCAP. This material is based upon work performed at the Joint Center for Artificial Photosynthesis (JCAP), a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. S.A. acknowledges support from the U.S. Department of Energy under Award No. DEEE0006963. | ||||||||||||||||||||||||||
| Group: | JCAP | ||||||||||||||||||||||||||
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| Subject Keywords: | device architecture; hydrogen; modeling; photoelectrochemistry; solar-driven water splitting | ||||||||||||||||||||||||||
| Issue or Number: | 42 | ||||||||||||||||||||||||||
| DOI: | 10.1002/anie.201510463 | ||||||||||||||||||||||||||
| Record Number: | CaltechAUTHORS:20160729-070531307 | ||||||||||||||||||||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20160729-070531307 | ||||||||||||||||||||||||||
| Official Citation: | C. Xiang, A. Z. Weber, S. Ardo, A. Berger, Y. Chen, R. Coridan, K. T. Fountaine, S. Haussener, S. Hu, R. Liu, N. S. Lewis, M. A. Modestino, M. M. Shaner, M. R. Singh, J. C. Stevens, K. Sun, K. Walczak, Angew. Chem. Int. Ed. 2016, 55, 12974 | ||||||||||||||||||||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | ||||||||||||||||||||||||||
| ID Code: | 69299 | ||||||||||||||||||||||||||
| Collection: | CaltechAUTHORS | ||||||||||||||||||||||||||
| Deposited By: | Ruth Sustaita | ||||||||||||||||||||||||||
| Deposited On: | 29 Jul 2016 16:44 | ||||||||||||||||||||||||||
| Last Modified: | 11 Nov 2021 04:12 |
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