Cheng, P. Y. and Zhong, D. and Zewail, Ahmed H. (1995) Kinetic-energy, femtosecond resolved reaction dynamics. Modes of dissociation (in iodobenzene) from time-velocity correlations. Chemical Physics Letters, 237 (5-6). pp. 399-405. ISSN 0009-2614. doi:10.1016/0009-2614(95)00364-A. https://resolver.caltech.edu/CaltechAUTHORS:20160825-105753554
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Abstract
We report on the use of ‘2D’ time-velocity correlations to study in real time the dynamics of reactions with multiple channels. By resolving the kinetic energy on the femtosecond time scale we are able to directly identify the direct-mode and complex-mode dissociation pathways of iodobenzene. The coherent wave packet dynamics and the nature of IVR in the benzen ring are discussed and related to the experimental observations.
| Item Type: | Article | |||||||||
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| Additional Information: | © 1995 Elsevier Science B.V. Received 6 March 1995. This work is supported by the National Science Foundation and the US Air Force Office of Scientific Research. We wish to thank Dr. J.K. Wang for his help in the initial setup of the fs laser system used in this work. We are grateful to the reviewer for his thorough reading of the manuscript. | |||||||||
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| Issue or Number: | 5-6 | |||||||||
| DOI: | 10.1016/0009-2614(95)00364-A | |||||||||
| Record Number: | CaltechAUTHORS:20160825-105753554 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20160825-105753554 | |||||||||
| Official Citation: | P.Y. Cheng, D. Zhong, Ahmed H. Zewail, Kinetic-energy, femtosecond resolved reaction dynamics. Modes of dissociation (in iodobenzene) from time-velocity correlations, Chemical Physics Letters, Volume 237, Issue 5, 1995, Pages 399-405, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(95)00364-A. (http://www.sciencedirect.com/science/article/pii/000926149500364A) | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 69932 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Ruth Sustaita | |||||||||
| Deposited On: | 26 Aug 2016 15:44 | |||||||||
| Last Modified: | 11 Nov 2021 04:22 |
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