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Rotational constants of vibrationally excited iodine from purely rotational coherence observed in pump-probe experiments

Willberg, D. M. and Breen, J. J. and Gutmann, M. and Zewail, A. H. (1991) Rotational constants of vibrationally excited iodine from purely rotational coherence observed in pump-probe experiments. Journal of Physical Chemistry, 95 (19). pp. 7136-7138. ISSN 0022-3654 . https://resolver.caltech.edu/CaltechAUTHORS:20160830-102557022

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Abstract

Pump-probe laser-induced fluorescence techniques are used to determine the rotational constants of vibrationally excited iodine, cooled by supersonic beam expansions. For comparison, it is shown that the results obtained from real time (purely rotational coherence) are in excellent agreement with literature values for the v' = 12-23 of the B state. Results for nascent I_2 (v' = 22), from the predissociation of I_2Ne (v' = 23), are also reported.


Item Type:Article
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http://dx.doi.org/10.1021/j100172a010DOIArticle
http://pubs.acs.org/doi/abs/10.1021/j100172a010PublisherArticle
Additional Information:© 1991 American Chemical Society. Received: July 12, 1991; In Final Form: August 8, 1991. This work was supported by a grant from the National Science Foundation.
Funders:
Funding AgencyGrant Number
NSFUNSPECIFIED
Other Numbering System:
Other Numbering System NameOther Numbering System ID
Arthur Amos Noyes Laboratory of Chemical Physics8474
Issue or Number:19
Record Number:CaltechAUTHORS:20160830-102557022
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20160830-102557022
Official Citation:Rotational constants of vibrationally excited iodine from purely rotational coherence observed in pump-probe experiments D. M. Willberg, J. J. Breen, M. Gutmann, and A. H. Zewail The Journal of Physical Chemistry 1991 95 (19), 7136-7138 DOI: 10.1021/j100172a010
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70026
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:31 Aug 2016 04:07
Last Modified:03 Oct 2019 10:27

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