Bowman, R. M. and Dantus, M. and Zewail, A. H. (1990) Femtosecond multiphoton dynamics of higher-energy potentials. Chemical Physics Letters, 174 (6). pp. 546-552. ISSN 0009-2614. doi:10.1016/0009-2614(90)85484-T. https://resolver.caltech.edu/CaltechAUTHORS:20160830-102642301
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Abstract
The real-time motion of wave packets prepared coherently in different potential energy surfaces of molecular iodine is reported. Using multiphoton excitation and depletion techniques, we observe the phase-shifted oscillatory motion of the packet and the different transients characteristic of the bound B 0^+u(^3Π) and D 0^+u(^1Σ) state potentials along with the repulsive 0^+g (^1Π) state potential. The approach helps in extending FTS to higher energy potentials and “dark” states, and illustrates experimental control schemes in a relatively simple system.
| Item Type: | Article | |||||||||
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| Additional Information: | © 1990 Elsevier Science Publishers 8.V. Received 30 August 1990; in final form 26 September 1990. This work was supported by the AFOSR. | |||||||||
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| Issue or Number: | 6 | |||||||||
| DOI: | 10.1016/0009-2614(90)85484-T | |||||||||
| Record Number: | CaltechAUTHORS:20160830-102642301 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20160830-102642301 | |||||||||
| Official Citation: | R.M. Bowman, M. Dantus, A.H. Zewail, Femtosecond multiphoton dynamics of higher-energy potentials, Chemical Physics Letters, Volume 174, Issue 6, 23 November 1990, Pages 546-552, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(90)85484-T. (http://www.sciencedirect.com/science/article/pii/000926149085484T) | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 70029 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Ruth Sustaita | |||||||||
| Deposited On: | 31 Aug 2016 01:07 | |||||||||
| Last Modified: | 11 Nov 2021 04:23 |
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