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Femtosecond multiphoton dynamics of higher-energy potentials

Bowman, R. M. and Dantus, M. and Zewail, A. H. (1990) Femtosecond multiphoton dynamics of higher-energy potentials. Chemical Physics Letters, 174 (6). pp. 546-552. ISSN 0009-2614. https://resolver.caltech.edu/CaltechAUTHORS:20160830-102642301

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Abstract

The real-time motion of wave packets prepared coherently in different potential energy surfaces of molecular iodine is reported. Using multiphoton excitation and depletion techniques, we observe the phase-shifted oscillatory motion of the packet and the different transients characteristic of the bound B 0^+u(^3Π) and D 0^+u(^1Σ) state potentials along with the repulsive 0^+g (^1Π) state potential. The approach helps in extending FTS to higher energy potentials and “dark” states, and illustrates experimental control schemes in a relatively simple system.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1016/0009-2614(90)85484-TDOIArticle
http://www.sciencedirect.com/science/article/pii/000926149085484TPublisherArticle
Additional Information:© 1990 Elsevier Science Publishers 8.V. Received 30 August 1990; in final form 26 September 1990. This work was supported by the AFOSR.
Funders:
Funding AgencyGrant Number
Air Force Office of Scientific Research (AFOSR)UNSPECIFIED
Other Numbering System:
Other Numbering System NameOther Numbering System ID
Arthur Amos Noyes Laboratory of Chemical Physics8211
Issue or Number:6
Record Number:CaltechAUTHORS:20160830-102642301
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20160830-102642301
Official Citation:R.M. Bowman, M. Dantus, A.H. Zewail, Femtosecond multiphoton dynamics of higher-energy potentials, Chemical Physics Letters, Volume 174, Issue 6, 23 November 1990, Pages 546-552, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(90)85484-T. (http://www.sciencedirect.com/science/article/pii/000926149085484T)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70029
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:31 Aug 2016 01:07
Last Modified:03 Oct 2019 10:27

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