Gruebele, M. and Roberts, G. and Dantus, M. and Bowman, R. M. and Zewail, A. H. (1990) Femtosecond temporal spectroscopy and direct inversion to the potential: Application to iodine. Chemical Physics Letters, 166 (5-6). pp. 459-469. ISSN 0009-2614. https://resolver.caltech.edu/CaltechAUTHORS:20160831-091534221
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Abstract
The use of femtosecond lasers in probing molecular dynamics is usually thought to yield improved temporal resolution, at the expense of spectral information. Here, we report on the use of femtosecond temporal spectroscopy (FTS) to yield accurate spectral information (vibrational and rotational) and to invert directly to the potential energy curve. As an example, we present the FTS analysis, inversion to the potential, and confirmatory wave packet calculations for the B ^3Π_(0+u) state of molecular iodine.
| Item Type: | Article | ||||||||||
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| Additional Information: | © 1990 Elsevier Science Publishers B.V. Received 19 January 1990. This work was supported by the National Science Foundation and the Air Force Office of Scientific Research. One of us (GR) thanks SERC for the award of a NATO Postdoctoral Fellowship. | ||||||||||
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| Issue or Number: | 5-6 | ||||||||||
| Record Number: | CaltechAUTHORS:20160831-091534221 | ||||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20160831-091534221 | ||||||||||
| Official Citation: | M. Gruebele, G. Roberts, M. Dantus, R.M. Bowman, A.H. Zewail, Femtosecond temporal spectroscopy and direct inversion to the potential: Application to iodine, Chemical Physics Letters, Volume 166, Issues 5–6, 9 March 1990, Pages 459-469, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(90)87134-D. (http://www.sciencedirect.com/science/article/pii/000926149087134D) | ||||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | ||||||||||
| ID Code: | 70060 | ||||||||||
| Collection: | CaltechAUTHORS | ||||||||||
| Deposited By: | Ruth Sustaita | ||||||||||
| Deposited On: | 31 Aug 2016 16:55 | ||||||||||
| Last Modified: | 03 Oct 2019 10:27 |
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