Vreeker, R. and Glasbeek, M. and Zewail, A. H. (1989) Photon locking and its observation by the probe-echo method: application to optical and microwave transitions. Journal of Physical Chemistry, 93 (2). pp. 658-664. ISSN 0022-3654. doi:10.1021/j100339a032. https://resolver.caltech.edu/CaltechAUTHORS:20160902-131818795
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Abstract
In this paper we consider the coherences that are produced in a photon (or spin) locking experiment involving a molecular two-level system. New coherences, not anticipated from the Feynman-Vernon-Hellwarth representation, are predicted if the transition is inhomogeneously broadened. The influence of duration, power, and phase of the driving and probe pulses in the locking experiment on the shape of the simulated echo responses is discussed in detail, and a comparison with experiments is made.
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| Additional Information: | © 1989 American Chemical Society. Received: June 20, 1988. This work was supported in part by the John van Geunsfonds and the United States National Science Foundation (Grant No. DMR 8521191). | |||||||||
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| Issue or Number: | 2 | |||||||||
| DOI: | 10.1021/j100339a032 | |||||||||
| Record Number: | CaltechAUTHORS:20160902-131818795 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20160902-131818795 | |||||||||
| Official Citation: | Photon locking and its observation by the probe-echo method: application to optical and microwave transitions R. Vreeker, M. Glasbeek, and A. H. Zewail The Journal of Physical Chemistry 1989 93 (2), 658-664 DOI: 10.1021/j100339a032 | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 70155 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Ruth Sustaita | |||||||||
| Deposited On: | 06 Sep 2016 19:11 | |||||||||
| Last Modified: | 11 Nov 2021 04:25 |
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