Baskin, J. S. and Dantus, M. and Zewail, A. H. (1986) Real-time measurements of IVR versus inferences from spectral broadening data: the alkylanilines “ring + tail” system. Chemical Physics Letters, 130 (6). pp. 473-481. ISSN 0009-2614. http://resolver.caltech.edu/CaltechAUTHORS:20160920-093337135
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Abstract
We report on picosecond/molecular beam studies of alkylanilines. The studies reveal important discrepancies between real-time measurements and inferences from spectral broadening data. We observe quantum recurrences and we find that the observed severe spectral congestion does not correspond to the observed coherence. The effect of mode symmetry and energy on IVR dynamics is also examined.
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| Additional Information: | © 1986 Elsevier B.V. Received 19 August 1986, in final form 27 August 1986. This work is supported by the National Science Foundation under Grant CHE-8512887. We wish to thank the group of Professor W.A. Goddard III for helping us to produce fig. 1 and Professor R.B. Bernstein for very helpful suggestions. | |||||||||
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| Record Number: | CaltechAUTHORS:20160920-093337135 | |||||||||
| Persistent URL: | http://resolver.caltech.edu/CaltechAUTHORS:20160920-093337135 | |||||||||
| Official Citation: | J.S. Baskin, M. Dantus, A.H. Zewail, Real-time measurements of IVR versus inferences from spectral broadening data: the alkylanilines “ring + tail” system, Chemical Physics Letters, Volume 130, Issue 6, 24 October 1986, Pages 473-481, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(86)80242-1. (http://www.sciencedirect.com/science/article/pii/0009261486802421) | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 70458 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Ruth Sustaita | |||||||||
| Deposited On: | 29 Sep 2016 21:17 | |||||||||
| Last Modified: | 29 Sep 2016 21:17 |
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