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Locking of Dephasing and Energy Redistribution in Molecular Systems by Multiple-Pulse Laser Excitation

Sleva, Edward T. and Glasbeek, Max and Zewail, Ahmed H. (1986) Locking of Dephasing and Energy Redistribution in Molecular Systems by Multiple-Pulse Laser Excitation. Journal of Physical Chemistry, 90 (7). pp. 1232-1234. ISSN 0022-3654. https://resolver.caltech.edu/CaltechAUTHORS:20160920-105242570

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Abstract

In this paper, we report experimental results on the locking of dephasing of molecules in the gas phase. The locking of inhomogeneous dephasing of the B ← X transition of iodine is achieved by using multiple-pulse and phase-coherent laser excitation, instead of a single-pulse excitation. We detect the locking using echo techniques. The locking concept is extended to the problem of intramolecular dephasing, emphasizing the potential for controlling selectivity in laser chemistry.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1021/j100398a007DOIArticle
http://pubs.acs.org/doi/abs/10.1021/j100398a007PublisherArticle
Additional Information:© 1986 American Chemical Society. Received: January 23, 1986. This work is supported by a grant from the National Science Foundation (DMR-8521191). M.G. and A.H.Z. also greatly acknowledge support from a NATO research grant.
Funders:
Funding AgencyGrant Number
NSFDMR-8521191
North Atlantic Treaty Organization (NATO)UNSPECIFIED
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Arthur Amos Noyes Laboratory of Chemical Physics7360
Issue or Number:7
Record Number:CaltechAUTHORS:20160920-105242570
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20160920-105242570
Official Citation:Locking of dephasing and energy redistribution in molecular systems by multiple-pulse laser excitation Edward T. Sleva, Ahmed H. Zewail, and Max Glasbeek The Journal of Physical Chemistry 1986 90 (7), 1232-1234 DOI: 10.1021/j100398a007
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70463
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:30 Sep 2016 17:51
Last Modified:03 Oct 2019 10:31

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