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Rephasing of Collisionless Molecular Rotational Coherence in Large Molecules

Felker, P. M. and Baskin, J. S. and Zewail, A. H. (1986) Rephasing of Collisionless Molecular Rotational Coherence in Large Molecules. Journal of Physical Chemistry, 90 (5). pp. 724-728. ISSN 0022-3654. doi:10.1021/j100277a006.

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We present experimental results on the rephasing of collisionless rotational coherence in jet-cooled trans-stitbene. The results represent the first observation of quantum coherence effects arising from the rotational level structure of molecules. We discuss the nature of the effect, its possible influence in time-resolved polarization experiments designed to probe intramolecular energy flow, and its possible uses as a new spectroscopic tool.

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Additional Information:© 1986 American Chemical Society. Received: January 3, 1986. We thank the National Science Foundation for support of this work through Grant No. DMR-8521191.
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Arthur Amos Noyes Laboratory of Chemical Physics7354
Issue or Number:5
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Official Citation:Rephasing of collisionless molecular rotational coherence in large molecules P. M. Felker, J. S. Baskin, and A. H. Zewail The Journal of Physical Chemistry 1986 90 (5), 724-728 DOI: 10.1021/j100277a006
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70464
Deposited By: Ruth Sustaita
Deposited On:30 Sep 2016 18:47
Last Modified:11 Nov 2021 04:29

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