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Picosecond saturation spectroscopy of cresyl violet: rotational diffusion by a “sticking” boundary condition in the liquid phase

Millar, D. P. and Shah, R. and Zewail, A. H. (1979) Picosecond saturation spectroscopy of cresyl violet: rotational diffusion by a “sticking” boundary condition in the liquid phase. Chemical Physics Letters, 66 (3). pp. 435-440. ISSN 0009-2614. http://resolver.caltech.edu/CaltechAUTHORS:20160927-092954082

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Abstract

Picosecond pulses (0.6–2.5 ps duration) from a passively mode-locked and cavity-dumped dye laser have been used to study the molecular reorientation of cresyl violet in liquids. The dipole correlation function is obtained from the decay of the induced dichroism. The results when compared with hydrodynamics give good agreement with the stick boundary condition, and predict effective shape of cresyl violet in the liquid.


Item Type:Article
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URLURL TypeDescription
http://dx.doi.org/10.1016/0009-2614(79)80311-510.1016/0009-2614(79)80311-5DOIArticle
http://www.sciencedirect.com/science/article/pii/0009261479803115PublisherArticle
Additional Information:© 1979 Elsevier B.V. Received 10 July 1979. We would like to thank the National Science Foundation and the United States Department of Energy.
Funders:
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NSFUNSPECIFIED
Department of Energy (DOE)UNSPECIFIED
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Arthur Amos Noyes Laboratory of Chemical Physics6053
Record Number:CaltechAUTHORS:20160927-092954082
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20160927-092954082
Official Citation:D.P. Millar, R. Shah, A.H. Zewail, Picosecond saturation spectroscopy of cresyl violet: rotational diffusion by a “sticking” boundary condition in the liquid phase, Chemical Physics Letters, Volume 66, Issue 3, 15 October 1979, Pages 435-440, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(79)80311-5. (http://www.sciencedirect.com/science/article/pii/0009261479803115)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70596
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:28 Sep 2016 23:11
Last Modified:02 Oct 2017 17:24

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