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Optical dephasing of small and large molecules: coherent oscillations of emitting molecules

Orlowski, T. E. and Jones, K. E. and Zewail, A. H. (1977) Optical dephasing of small and large molecules: coherent oscillations of emitting molecules. Chemical Physics Letters, 50 (1). pp. 45-50. ISSN 0009-2614. http://resolver.caltech.edu/CaltechAUTHORS:20160927-112618716

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Abstract

We describe the conditions under which large and small molecules may undergo optical dephasing. The relationship between the coherent preparation of excited states and the intramolecular and intermolecular processes are discussed and related to the recent measurements of optical T_1 and T_2. Finally, we report on the observation of a coherent (oscillatory) transient on the spontaneous emission of iodine gas.


Item Type:Article
Related URLs:
URLURL TypeDescription
http://dx.doi.org/10.1016/0009-2614(77)80677-5DOIArticle
http://www.sciencedirect.com/science/article/pii/0009261477806775PublisherArticle
Additional Information:© 1977 Elsevier B.V. Received 9 May 1977. Acknowledgement is made to the donors of the Petroleum Research Fund, administered by the ACS, for partial support of this research. This work was also supported in part by the Research Corporation. We would like to thank J. Jortner for the critical reading of the manuscript and for very stimulating discussions.
Funders:
Funding AgencyGrant Number
American Chemical Society Petroleum Research FundUNSPECIFIED
Research CorporationUNSPECIFIED
Other Numbering System:
Other Numbering System NameOther Numbering System ID
Arthur Amos Noyes Laboratory of Chemical Physics5585
Record Number:CaltechAUTHORS:20160927-112618716
Persistent URL:http://resolver.caltech.edu/CaltechAUTHORS:20160927-112618716
Official Citation:T.E. Orlowski, K.E. Jones, A.H. Zewail, Optical dephasing of small and large molecules: coherent oscillations of emitting molecules, Chemical Physics Letters, Volume 50, Issue 1, 15 August 1977, Pages 45-50, ISSN 0009-2614, http://dx.doi.org/10.1016/0009-2614(77)80677-5. (http://www.sciencedirect.com/science/article/pii/0009261477806775)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:70607
Collection:CaltechAUTHORS
Deposited By: Ruth Sustaita
Deposited On:28 Sep 2016 23:01
Last Modified:28 Sep 2016 23:01

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