Jones, K. E. and Zewail, A. H. and Diestler, D. J. (1978) Molecular Mechanisms for Dephasing: Toward a Unified Treatment of Gases, Solids and Liquids. In: Advances in Laser Chemistry. Springer Series in Chemical Physics . No.3. Springer-Verlag , New York, NY, pp. 258-270. ISBN 978-3-642-67056-5. https://resolver.caltech.edu/CaltechAUTHORS:20161005-085505684
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Abstract
In this paper we are concerned with the role of dephasing (optical T_1 and T_2) in various molecular relaxation processes. Specifically, we are asking the following questions: (1) What is the relationship between the lineshape function and the dephasing time? (2) What are the different processes that contribute to the overall dephasing rate? (3) Are the approximations made in describing dephasing in solids and liquids reasonable ? (4) Can we use a unified theoretical approach to describe dephasing in gases, solids, and liquids?
| Item Type: | Book Section | |||||||||
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| Additional Information: | © 1978 Springer-Verlag Berlin Heidelberg. This work was supported in part by a grant from NSF to A. H. Zewail and D. J. Diestler. Acknowledgment is also made to the donors of the Petroleum Research Fund, administered by ACS, for partial support of this research (AHZ). | |||||||||
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| Series Name: | Springer Series in Chemical Physics | |||||||||
| Issue or Number: | 3 | |||||||||
| DOI: | 10.1007/978-3-642-67054-1_24 | |||||||||
| Record Number: | CaltechAUTHORS:20161005-085505684 | |||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20161005-085505684 | |||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | |||||||||
| ID Code: | 70861 | |||||||||
| Collection: | CaltechAUTHORS | |||||||||
| Deposited By: | Ruth Sustaita | |||||||||
| Deposited On: | 05 Oct 2016 18:30 | |||||||||
| Last Modified: | 11 Nov 2021 04:36 |
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