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Year-long simulation of gaseous and particulate air pollutants in India

Kota, Sri Harsha and Guo, Hao and Myllyvirta, Lauri and Hu, Jianlin and Sahu, Shovan Kumar and Garaga, Rajyalakshmi and Ying, Qi and Gao, Aifang and Dahiya, Sunil and Wang, Yuan and Zhang, Hongliang (2018) Year-long simulation of gaseous and particulate air pollutants in India. Atmospheric Environment, 180 . pp. 244-255. ISSN 1352-2310 . https://resolver.caltech.edu/CaltechAUTHORS:20180509-090908650

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Abstract

Severe pollution events occur frequently in India but few studies have investigated the characteristics, sources, and control strategies for the whole country. A year-long simulation was carried out in India to provide detailed information of spatial and temporal distribution of gas species and particulate matter (PM). The concentrations of O_3, NO_2, SO_2, CO, as well as PM_(2.5) and its components in 2015 were predicted using Weather Research Forecasting (WRF) and the Community Multiscale Air Quality (CMAQ) models. Model performance was validated against available observations from ground based national ambient air quality monitoring stations in major cities. Model performance of O_3 does not always meet the criteria suggested by the US Environmental Protection Agency (EPA) but that of PM_(2.5) meets suggested criteria by previous studies. The performance of model was better on days with high O_3 and PM_(2.5) levels. Concentrations of PM_(2.5), NO_2, CO and SO_2 were highest in the Indo-Gangetic region, including northern and eastern India. PM_(2.5) concentrations were higher during winter and lower during monsoon season. Winter nitrate concentrations were 160–230% higher than yearly average. In contrast, the fraction of sulfate in total PM_(2.5) was maximum in monsoon and least in winter, due to decrease in temperature and solar radiation intensity in winter. Except in southern India, where sulfate was the major component of PM_(2.5), primary organic aerosol (POA) fraction in PM_(2.5) was highest in all regions of the country. Fractions of secondary components were higher on bad days than on good days in these cities, indicating the importance of control of precursors for secondary pollutants in India.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1016/j.atmosenv.2018.03.003DOIArticle
ORCID:
AuthorORCID
Wang, Yuan0000-0001-6657-8401
Additional Information:© 2018 Elsevier Ltd. Received 19 September 2017, Revised 21 January 2018, Accepted 3 March 2018, Available online 5 March 2018. Portions of this research were conducted with high performance computing resources provided by Louisiana State University (http://www.hpc.lsu.edu) and Indian Institute of Technology, Guwahati (http://www.iitg.ernet.in/param-ishan/index.html). The project is funded by European Climate Foundation (G-1606-00917). Open fund by Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control (KHK1512), A Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD).
Funders:
Funding AgencyGrant Number
European Climate FoundationG-1606-00917
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlKHK1512
Jiangsu Higher Education InstitutionsUNSPECIFIED
Subject Keywords:Ozone; Particulate matter; WRF; CMAQ; EDGAR; India
Record Number:CaltechAUTHORS:20180509-090908650
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20180509-090908650
Official Citation:Sri Harsha Kota, Hao Guo, Lauri Myllyvirta, Jianlin Hu, Shovan Kumar Sahu, Rajyalakshmi Garaga, Qi Ying, Aifang Gao, Sunil Dahiya, Yuan Wang, Hongliang Zhang, Year-long simulation of gaseous and particulate air pollutants in India, Atmospheric Environment, Volume 180, 2018, Pages 244-255, ISSN 1352-2310, https://doi.org/10.1016/j.atmosenv.2018.03.003. (http://www.sciencedirect.com/science/article/pii/S1352231018301419)
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:86305
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:09 May 2018 16:36
Last Modified:03 Oct 2019 19:42

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