Vanelderen, Pieter and Hadt, Ryan G. and Smeets, Pieter J. and Solomon, Edward I. and Schoonheydt, Robert A. and Sels, Bert F. (2011) Cu-ZSM-5: A biomimetic inorganic model for methane oxidation. Journal of Catalysis, 284 (2). pp. 157-164. ISSN 0021-9517. PMCID PMC3593946. doi:10.1016/j.jcat.2011.10.009. https://resolver.caltech.edu/CaltechAUTHORS:20180612-134854687
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Abstract
The present work highlights recent advances in elucidating the methane oxidation mechanism of inorganic Cu-ZSM-5 biomimic and in identifying the reactive intermediates that are involved. Such molecular understanding is important in view of upgrading abundantly available methane, but also to comprehend the working mechanism of genuine Cu-containing oxidation enzymes.
| Item Type: | Article | ||||||||||
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| Additional Information: | © 2011 Elsevier. Available online 14 November 2011. This work was performed within the framework of FWO (G.0596.11), IAP (Belspo), ERIC and Methusalem (long-term structural funding by the Flemish Government) projects. E.I.S. acknowledges the NIH (Grant DK-31450), and R.G.H. acknowledges a Gerhard Casper Stanford Graduate Fellowship. | ||||||||||
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| Subject Keywords: | Zeolite, Cu-ZSM-5, Dioxygen activation, Dicopper(II) oxo, Model complex, Selective methane oxidation, C-H activation | ||||||||||
| Issue or Number: | 2 | ||||||||||
| PubMed Central ID: | PMC3593946 | ||||||||||
| DOI: | 10.1016/j.jcat.2011.10.009 | ||||||||||
| Record Number: | CaltechAUTHORS:20180612-134854687 | ||||||||||
| Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20180612-134854687 | ||||||||||
| Official Citation: | Pieter Vanelderen, Ryan G. Hadt, Pieter J. Smeets, Edward I. Solomon, Robert A. Schoonheydt, Bert F. Sels, Cu-ZSM-5: A biomimetic inorganic model for methane oxidation, Journal of Catalysis, Volume 284, Issue 2, 2011, Pages 157-164, ISSN 0021-9517, https://doi.org/10.1016/j.jcat.2011.10.009. (http://www.sciencedirect.com/science/article/pii/S0021951711003435) | ||||||||||
| Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | ||||||||||
| ID Code: | 87016 | ||||||||||
| Collection: | CaltechAUTHORS | ||||||||||
| Deposited By: | George Porter | ||||||||||
| Deposited On: | 12 Jun 2018 21:03 | ||||||||||
| Last Modified: | 15 Nov 2021 20:44 |
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