Mead, Griffin and Katayama, Ikufumi and Takeda, Jun and Blake, Geoffrey A. (2019) An echelon-based single shot optical and terahertz Kerr effect spectrometer. Review of Scientific Instruments, 90 (5). Art. No. 053107. ISSN 0034-6748. PMCID PMC6842322. doi:10.1063/1.5088377. https://resolver.caltech.edu/CaltechAUTHORS:20190520-081811604
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Abstract
We report on the design and performance of an echelon-based single shot visible/near-infrared spectrometer with adequate sensitivity to measure the nonlinear optical and terahertz Kerr effects in neat molecular liquids at room temperature. Useful molecular information spanning tens of picoseconds can be measured in just a few milliseconds, and the signal-to-noise performance scales favorably with respect to the standard stage scan technique. These results demonstrate the viability of stage-free nonlinear Kerr effect measurements and provide a route for improvements to the speed of future multidimensional Kerr effect studies.
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Additional Information: | © 2019 Published under license by AIP Publishing. Submitted: 9 January 2019; Accepted: 21 April 2019; Published Online: 13 May 2019. This research is based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE 1745301. This research was further supported by grants from the National Science Foundation Chemical Structure, Dynamics, and Mechanisms program (Grant No. CHE-1665467), from the National Aeronautics and Space Administration Astrophysics Research and Analysis (Grant No. NNX16AC75G) and Astrobiology (Grant No. NNX15AT33A) programs, and from the Grants-in-Aid for Scientific Research (Grant Nos. 18H04288, 16H04001, and 17H06124) from the Ministry of Sports, Culture, Science, and Technology, Japan. | ||||||||||||||||
Group: | Astronomy Department | ||||||||||||||||
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Issue or Number: | 5 | ||||||||||||||||
PubMed Central ID: | PMC6842322 | ||||||||||||||||
DOI: | 10.1063/1.5088377 | ||||||||||||||||
Record Number: | CaltechAUTHORS:20190520-081811604 | ||||||||||||||||
Persistent URL: | https://resolver.caltech.edu/CaltechAUTHORS:20190520-081811604 | ||||||||||||||||
Usage Policy: | No commercial reproduction, distribution, display or performance rights in this work are provided. | ||||||||||||||||
ID Code: | 95585 | ||||||||||||||||
Collection: | CaltechAUTHORS | ||||||||||||||||
Deposited By: | Tony Diaz | ||||||||||||||||
Deposited On: | 20 May 2019 16:16 | ||||||||||||||||
Last Modified: | 16 Nov 2021 17:13 |
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