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The Spider DMA: A miniature radial differential mobility analyzer

Amanatidis, Stavros and Kim, Changhyuk and Spielman, Steven R. and Lewis, Gregory S. and Hering, Susanne V. and Flagan, Richard C. (2020) The Spider DMA: A miniature radial differential mobility analyzer. Aerosol Science and Technology, 54 (2). pp. 175-189. ISSN 0278-6826. doi:10.1080/02786826.2019.1626974. https://resolver.caltech.edu/CaltechAUTHORS:20190624-074058334

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Abstract

The Spider differential mobility analyzer (DMA) is a novel, miniaturized radial DMA developed to provide size classification in the 10–500 nm range for applications requiring high portability and time resolution. Its external dimensions are ∼12 cm in diameter by 6 cm in height (excluding tubing); it weighs ∼350 g, and is designed to operate at 0.6–1.5 L/min sheath and 0.3 L/min sample flowrates. It features a new sample inlet geometry that is designed to produce a uniform azimuthal particle distribution at the entrance of the classifier, optimized sample/sheath flow streams introduction in the classifier to minimize particle delays, and extension of the electric field interaction volume for ∼30% enhanced dynamic range. Based on three-dimensional finite element simulations of flows, electric fields, and particle trajectories, we demonstrate that the Spider DMA transfer functions can be predicted with high fidelity using a parameterized fit based on the Stolzenburg semi-analytical model. Experimental characterization of the instrument response with size-selected particles confirmed close agreement with model prediction; mobility size response is linear over three orders of magnitude in mobility span. Electrical ground shielding of the external surfaces of the DMA has been found to be necessary to avoid particle losses associated with field effects as the high voltage operating limit is approached. The mean deviation between the reference size of polystyrene latex spheres and the Spider DMA measurement is less than 2%, corroborating its high sizing precision and potential for high quality size distribution measurements.


Item Type:Article
Related URLs:
URLURL TypeDescription
https://doi.org/10.1080/02786826.2019.1626974DOIArticle
ORCID:
AuthorORCID
Amanatidis, Stavros0000-0002-4924-8424
Kim, Changhyuk0000-0002-8744-4880
Flagan, Richard C.0000-0001-5690-770X
Additional Information:© 2019 American Association for Aerosol Research. Received 02 Mar 2019, Accepted 26 May 2019, Accepted author version posted online: 07 Jun 2019, Published online: 19 Jun 2019. The authors would like to thank Dr. Huajun Mai for helpful discussions and assistance in preparation of the experimental data acquisition software. This research was supported by the Small Business Innovative Research and Small Business Technology Transfer Department of Energy Research Grant No. DE-SC0013152.
Funders:
Funding AgencyGrant Number
Department of Energy (DOE)DE-SC0013152
Issue or Number:2
DOI:10.1080/02786826.2019.1626974
Record Number:CaltechAUTHORS:20190624-074058334
Persistent URL:https://resolver.caltech.edu/CaltechAUTHORS:20190624-074058334
Official Citation:Stavros Amanatidis, Changhyuk Kim, Steven R. Spielman, Gregory S. Lewis, Susanne V. Hering & Richard C. Flagan (2020) The Spider DMA: A miniature radial differential mobility analyzer, Aerosol Science and Technology, 54:2, 175-189, DOI: 10.1080/02786826.2019.1626974
Usage Policy:No commercial reproduction, distribution, display or performance rights in this work are provided.
ID Code:96647
Collection:CaltechAUTHORS
Deposited By: Tony Diaz
Deposited On:24 Jun 2019 17:07
Last Modified:16 Nov 2021 17:22

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