Published January 19, 2024 | Version Published
Journal Article Open

Sympathetic Cooling and Slowing of Molecules with Rydberg Atoms

Abstract

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize the molecules even in a low-density environment. Molecules traveling at 100m/s can be stopped in under 30 collisions with little inelastic loss. Our method does not require photon scattering from the molecules and can be generically applied to complex species for applications in precision measurement, quantum information science, and controlled chemistry.

Copyright and License

© 2024 American Physical Society.

Acknowledgement

Files

PhysRevLett.132.033001.pdf

Files (973.7 kB)

Name Size Download all
md5:54e1736bb5a0f2356788d8f71ad04965
702.1 kB Preview Download
md5:306f9449293fee0636ceaef8906a70d2
271.6 kB Preview Download

Additional details

Identifiers

ISSN
1079-7114

Funding

Gordon and Betty Moore Foundation
GBMF7947
Alfred P. Sloan Foundation
G-2019-12502
California Institute of Technology
David and Ellen Lee Postdoctoral Fellowship
National Science Foundation
PHY-2045681
Harvard University

Caltech Custom Metadata

Caltech groups
Institute for Quantum Information and Matter