Particle composition measurements during CLOUD7
Abstract
The chemical composition of >8 nm diameter aerosol was measured using the Timeof-Flight Thermal Desorption Chemical Ionization Mass Spectrometer (TOF-TDCIMS) during CLOUD7 particle nucleation experiments in Fall 2012 at the CLOUD chamber at CERN in Geneva, Switzerland. Sulfate dominated the negative ion particle spectra during all events with enough particle mass to observe, both in experiments with amine and alpha-pinene. Ammonium was also a major particle constituent during all observable events, though gaseous ammonia was present in the chamber only as a contaminant. During nucleation events following the oxidation of alpha-pinene, highly oxidized organic acids such as oxalic and oxoacetic acid were observed to be significant components of the collected aerosol.
Additional Information
© 2013 AIP Publishing LLC. Published online 24 May 2013. We would like to thank CERN for supporting CLOUD with important technical and financial resources, and for providing a particle beam from the CERN Proton Synchrotron. This research has received funding from the EC Seventh Framework Programme (Marie Curie Initial Training Network "CLOUD-ITN" no. 215072, MCITN "CLOUD-TRAIN" no. 316662, and ERC-Advanced "ATMNUCLE'' grant no. 227463), the German Federal Ministry of Education and Research (project nos. 01LK0902A and 01LK1222A), the Swiss National Science Foundation (project nos. 200020_135307 and 206620_130527), the Academy of Finland (Center of Excellence project no. 1118615), the Academy of Finland (135054, 133872, 251427, 139656, 139995, 137749, 141217, 141451), the Finnish Funding Agency for Technology and Innovation, the Nessling Foundation, the Austrian Science Fund (FWF; project no. P19546 and L593), the Portuguese Foundation for Science and Technology (project no. CERN/FP/116387/2010), the Swedish Research Council, Vetenskapsrådet (grant 2011-5120), the Presidium of the Russian Academy of Sciences and Russian Foundation for Basic Research (grants 08-02-91006-CERN and 12-02-91522-CERN), and the U.S. National Science Foundation (grants AGS1136479 and CHE1012293).Attached Files
Published - 1.4803284.pdf
Files
Name | Size | Download all |
---|---|---|
md5:29dd94b9d4b9dc90b482e50f6be504e3
|
724.6 kB | Preview Download |
Additional details
- Eprint ID
- 66340
- Resolver ID
- CaltechAUTHORS:20160420-155739931
- Marie Curie Fellowship
- 215072
- Marie Curie Fellowship
- 316662
- European Research Council (ERC)
- 227463
- Bundesministerium für Bildung und Forschung (BMBF)
- 01LK0902A
- Bundesministerium für Bildung und Forschung (BMBF)
- 01LK1222A
- Swiss National Science Foundation (SNSF)
- 200020_135307
- Swiss National Science Foundation (SNSF)
- 206620_130527
- Academy of Finland
- 1118615
- Academy of Finland
- 135054
- Academy of Finland
- 133872
- Academy of Finland
- 251427
- Academy of Finland
- 139656
- Academy of Finland
- 139995
- Academy of Finland
- 137749
- Academy of Finland
- 141217
- Academy of Finland
- 141451
- Finnish Funding Agency for Technology and Innovation
- Nessling Foundation
- FWF Der Wissenschaftsfonds
- P19546
- FWF Der Wissenschaftsfonds
- L593
- Fundação para a Ciência e a Tecnologia (FCT)
- CERN/FP/116387/2010
- Swedish Research Council
- Vetenskapsrådet
- 2011-5120
- Russian Academy of Sciences
- Russian Foundation for Basic Research
- 08-02-91006-CERN
- Russian Foundation for Basic Research
- 12-02-91522-CERN
- NSF
- AGS1136479
- NSF
- CHE1012293
- Created
-
2016-04-20Created from EPrint's datestamp field
- Updated
-
2021-11-10Created from EPrint's last_modified field
- Series Name
- AIP Conference Proceedings
- Series Volume or Issue Number
- 1527