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Published December 8, 1999 | Published
Journal Article Open

On the direct evaluation of the equilibrium distribution of clusters by simulation


An expression is derived that relates the average population of a particular type of cluster in a metastable vapor phase of volume Vtot to the probability, estimated by simulation, of finding this cluster in a system of volume V taken inside Vtot, where V<

Additional Information

Copyright © 1999 American Institute of Physics. (Received 22 April 1999; accepted 31 August 1999) This work was supported by the National Science Foundation (Grant No. CHE-9800074). Z.-G.W. acknowledges support from the Camille and Henry Dreyfus Foundation, the Alfred P. Sloan Foundation, the National Science Foundation and a Grant by the Mobil Corporation.

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