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Published December 15, 1990 | Published
Journal Article Open

Direct observation of the picosecond dynamics of I_2-Ar fragmentation


Picosecond real‐time observations of the dynamics of I_2–Ar fragmentation are reported. The state‐to‐state rates, k(ν^i,,ν^f,), are directly measured and related to the homogeneous broadening of the initial state, and to product state distributions in the exit channel. Comparisons with different theories of vibrational (and electronic) predissociation are made.

Additional Information

© 1990 American Institute of Physics. Received 27 August 1990; accepted 3 October 1990. This work was supported by the National Science Foundation.

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