Atoms as nonlinear mixers for detection of quantum correlations at ultrahigh frequencies

Measurements of quantum correlations are reported for a frequency difference of 25 THz between the signal and idler output fields generated by a subthreshold nondegenerate optical parametric oscillator. By simultaneously exciting a two-photon transition in atomic Cs by a combination of signal, idler, and "references oscillator" fields, we record modulation of the excited-state population due to quantum interference between two alternative excitation pathways. The observed phase-sensitive modulation is proportional to the correlation function〈EsEi〉for the quantized signal and idler fields.